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IEEE TRANSACTIONS ON ANTENNAS AND PROPAGATION, VOL. 59, NO. 9, SEPTEMBER 2011
I. INTRODUCTION
HE quest for miniaturization, integration, higher compactness, and speed in circuit devices, is leading towards
ever higher and higher frequency regimes. This trend gave
way from microwave to terahertz, and more lately to optical
frequency regimes. However, metal dispersive properties at
optical frequencies present a new challenge in the electromagnetic modeling of such devices, as a direct scaling from
lower frequency bands is no longer possible and thus a proper
review is required. In these regimes the interaction of free
light with the electron bulk sea in the metals surface gives
Manuscript received July 09, 2010; revised January 19, 2011; accepted
January 31, 2011. Date of publication July 12, 2011; date of current version September 02, 2011. This work was supported in part by the Flemish
government through the Methusalem framework and in part by the Fonds
Wetenschappelijk Onderzoek Vlaanderen (FWO) through several research
projects.
F. P. G. de Arquer was with the Katholieke Universiteit Leuven,
ESAT-TELEMIC, 3001 Leuven, Belgium. He is now with the Institute
of Photonic Sciences, 08860 Barcelona, Spain (e-mail: pelayo.garciadearquer@icfo.es).
V. Volski, and G. A. E. Vandenbosch are with the Katholieke Universiteit Leuven, ESAT-TELEMIC, 3001 Leuven, Belgium (e-mail:
vladimir.volski@esat.kuleuven.be; guy.vandenbosch@esat.kuleuven.be).
N. Verellen is with the Katholieke Universiteit Leuven, ESAT-TELEMIC; Institute for Nanoscale Physics and Chemistry, Nanoscale Superconductivity and
Magnetism and Pulsed Fields Group; IMEC, 3001, Leuven, Belgium (e-mail:
Niels.Verellen@fys.kuleuven.be).
V. V. Moshchalkov is with the Institute for Nanoscale Physics and Chemistry,
Nanoscale Superconductivity and Magnetism and Pulsed Fields Group, 3001
Leuven, Belgium (e-mail: victor.moshchalkov@fys.kuleuven.be).
Color versions of one or more of the figures in this paper are available online
at http://ieeexplore.ieee.org.
Digital Object Identifier 10.1109/TAP.2011.2161544
DE ARQUER et al.: ENGINEERING THE INPUT IMPEDANCE OF OPTICAL NANO DIPOLE ANTENNAS
should also be included in further antenna analysis and characterization. In this paper, the input impedance of a gap fed
nano dipole antenna is analyzed for several metal and substrate
materials, in a two semi infinite media environment that models
the effect of the substrate, for varying antenna length and
width. These results are compared with the behavior of radio
frequency (RF) antennas, where the dispersive properties of the
metals are negligible. A linear model of the resonant response
of the antennas is established. This is very useful in designs as
it can take advantage of all the knowledge in antenna theory
acquired at lower frequencies. After this study a comparison
of gap fed excitation with plane wave excitation is performed.
The optical cross sections, corresponding to the plane wave
excitation, are determined. All the calculations were performed
with an in-house developed simulation tool, MAGMAS 3D
[24]. The simulation procedure is based on a combination
of surface and volume integral equations in a multilayered
environment. These equations are solved using the method of
moments (MoM). Surface currents are meshed using rectangles
and triangles and volume currents are meshed using hexahedra.
Additional details about the used techniques can be found in
[25][28].
This tool was originally developed for the microwave regime
and extended considerably to the optical regime [29]. The MoM
technique [30] is known as a very powerful, robust, and fast
technique in classical antenna problems. In the optical domain
however, up to now it has been completely deprecated by the
finite elements method (FEM) or finite-difference time-domain
(FDTD) modeling technique, which is used in most commercial
solvers there. The main intrinsic strength of a MoM solver is the
much lower number of unknowns describing the problem. This
argument actually still holds also in the optical regime, as only
micro/nanostructures need to be discretized.
II. THEORY AND VALIDATION
The first great advantage of the MoM in comparison with the
FEM and the FDTD method is that only the current carrying
components (the dipoles) in Fig. 1 have to be discretized.
The complex environment, which may include multilayered
substrates, is taken into account via Greens functions. The
discretized components are modeled in terms of equivalent
currents. These currents fill completely all metal/dielectric
volumes and the boundary conditions are satisfied in an average
sense inside these volumes, on surfaces or lines depending
on the selected testing procedure. The result is that MoM is
intrinsically faster than the two other methods. The second
advantage of the MoM technique is that, if properly formulated,
it is variationally stable since most of the output parameters
are expressed in integral form over the equivalent currents.
As a consequence even if the calculated currents differ considerably from the exact solution, integral parameters over
both currents may remain very similar. Further, this will be
illustrated by showing that even with a rather rough mesh high
quality physical results may be obtained. A third advantage is
that MoM does not heavily suffer from field singularities near
sharp edges, since they are analytically incorporated inside the
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Fig. 1. (a) Schematic of the dipole antenna geometry and dimensions. (b)
Schematic of the excitation setup and input impedance retrieval. An imposed
current (red) is flowing over two passive patches (green) to the two dipole arms.
(c) Plane wave illumination.
Greens functions. For the FEM and the FDTD method special
) should be taken to describe correctly
care (
these field singularities.
The antenna design is based on the work of Muhlschlegel et
al. [12] where the optical response of plasmonic nano antennas
was studied. The geometry and defining parameters are depicted
,
and
.
in Fig. 1(a):
This structure is modeled in MAGMAS sandwiched between
two semi infinite media, one (the bottom) taken as substrate and
the other as vacuum. The dipole arms are meshed with 5 5 8
hexahedrons, which is optimal for this structure and increases also the efficiency of MoM by the use of translation
symmetry.
The extinction cross section of a gold monomer calculated using MAGMAS 3D with different meshes is plotted in
Fig. 2(a). The analysis of these data demonstrates clearly the
stability of the MoM [30]. The results obtained even with a very
rough mesh 6 1 1 (41.7 nm 40 nm 40 nm) provides
already a very good estimation of the antenna resonance properties. The differences in extinction cross section calculated with
the rough and fine meshes are almost negligibly small. On the
adjacent figure Fig. 2(b) extinction cross sections are calculated
using Lumerical [31], a commercial solver based on the FDTD
method. As expected, in general the results obtained with the
FDTD method depend considerably on the chosen mesh. A fine
mesh should be used for reliable calculations of the monomer
resonant wavelength. The calculated wavelengths as a function
of the mesh cell size are plotted in Fig. 3. It should be also noted
that in contrast to Fig. 2(a) (MoM) in Fig. 2(b) (FDTD) not only
peak positions but also their levels depend clearly on the mesh.
However, for both methods shown in Fig. 2, the convergence of
the numerical results is not an ultimate proof of the accuracy.
Comparison with the exact solution or experimental results still
remains a more convincing validation.
As a next step, several gold monomers with different lengths
were fabricated on a glass substrate by means of electron beam
lithography and ion-milling. The fabricated monomers have a
height and width of about 60 nm and 110 nm, respectively. The
maximal lengths of the monomers are 265 nm, 205 nm and
165 nm. A scanning electron microscopy (SEM) image of the
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IEEE TRANSACTIONS ON ANTENNAS AND PROPAGATION, VOL. 59, NO. 9, SEPTEMBER 2011
monomer with length 265 nm is shown in Fig. 4. As a consequence of the fabrication method the side walls of all particles have a slope of about 20 degrees. Extinction cross secwith 2
pitch were meations of arrays of 50 by 50
sured using a Fourier transform infrared spectrometer equipped
with a microscope. They are shown in Fig. 4. The monomers
were illuminated by a plane wave polarized along the longitudinal axis. Considering the fact that the distance between the
dipoles in the array is considerably larger than a wavelength,
in the case of normal incidence the response of a dipole in the
array is almost identical to the response of a single dipole. Regarding the electromagnetic modeling, in the case of Lumerical (FDTD method), the space was meshed in 5 nm side cubes
in a box surrounding the particle. The plane wave excitation
within MAGMAS illuminates the sample from the substrate
side, whereas in Lumerical it is top illuminated. This difference does not affect the obtained cross sections. The MAGMAS
mesh cell size is about 20 nm, i.e., 16 6 3 cells for 265 nm,
10 6 3 cells for 205 nm, and 9 6 3 cells for 165 nm.
The used complex permittivity of gold was taken from [32].
The substrate was modeled with a constant 1.5 refractive index.
In the case of the FDTD method the dielectric response of the
metal was fitted using the multicoefficient model of Lumerical
[31] that indeed offers a good fit to [32] (not shown here). Simulation values for both solvers were normalized and adjusted
to match the experiment. This change of scale does not affect
the interpretation of the results, because the important feature
here is the extinction shape. The agreement between them is evident, although both simulations are red-shifted with respect to
the measurements. These differences are partially due to the fact
that rectangular prisms were used in both simulations resulting
in larger monomer volumes in comparison with their real sizes
in the experiment.
III. GAP EXCITATION
An essential parameter of any receiving or transmitting antenna is its input impedance [33][36]. This parameter is absolutely needed in order to be able to describe the coupling between an antenna and the connected circuits, being part of a
receiver or transmitter, respectively. This is evident at RF and
DE ARQUER et al.: ENGINEERING THE INPUT IMPEDANCE OF OPTICAL NANO DIPOLE ANTENNAS
3147
venient since it drastically enhances return losses, therefore requiring a large impedance matching network. As the wavelength
gets closer to resonance, the reactance starts to behave induc) and the resistance starts to grow rapidly. The
tively (
crosses zero from negative to positive values
points where
show series LC resonant behavior. For those wavelengths the
input impedance is purely resistive, but still much smaller than
, at what can be seen as a short circuit resonance. For
gold this occurs at approximately 1225 nm for an arm length
, yielding
[Fig. 5(a)(b)]. This is
of
.
one order of magnitude smaller than
This resonance is the counterpart of the well known
for
thin RF dipoles. Going down in wavelength, close to the
maximum resistance resonance, the reactance crosses zero again
and now starts to behave capacitively (parallel LC resonant behavior). In these points the impedance is only resistive but larger
. For the same case
at 920 nm is obthan
tained. For longer wavelengths the reactance remains negative
and the resistance decays until second order resonances appear
at 565 nm). Be(in the same case
cause the resistance peak corresponds to maximum scattering
cross section or, equivalently, radiated power, dipole dimensions (or the working wavelength band) should be chosen as a
trade off between radiation efficiency and impedance matching,
both strongly relying on the feeding line properties [23]. For
other antenna materials the results are qualitatively similar. The
case of silver [Fig. 5(c)(d)] is blueshifted with respect to gold,
and presents also slightly smaller resistance values. For copper
[Fig. 5(e)(f)] the similarities with gold are remarkable. Although resistance values are a little bit higher for the second resonance (about 500 ), resonance positions only differ in a few
nanometers, opening up interesting design choices depending
on the environment. This fact is explained by the almost identical complex permittivity in the analyzed wavelengths for both
materials. The aluminium case [Fig. 5(g)(h)] presents a new
phenomenon with respect to the previous metals. An additional
at around 900
peak appears in the resistance for
nm, and also the reactance is shifted to negative values in a way
different from typical series and parallel LC resonances. This is
explained by the interband transitions that approximately occur
at this wavelength. The resistance is also much smaller, below
at maximum. Note that for all cases the resistance
1.5
and the impedance amplitude show a significant decrease as
dipole arms get shortened. This is caused by the bigger electrical size of the gap for each resonant frequency. The case of
PEC [Fig. 5(i)(j)] serves as a non dispersive reference, thus representing the RF down scaled equivalent. The overall response
is qualitatively similar, but a very clear and important differ) for the real metals
ence is noticed. Resonant positions (
are strongly redshifted with respect to the expected values in
classic antenna theory. The first one is traditionally given by
for thin dipoles. This phenomenon is properly explained by the dispersive properties of the metals at optical frequencies, which introduces an effective wavelength scaling in
the form of (1) [21]
(1)
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IEEE TRANSACTIONS ON ANTENNAS AND PROPAGATION, VOL. 59, NO. 9, SEPTEMBER 2011
Fig. 5. Input impedance as a function of when varying dipole arm length L in steps of 10 nm for different antenna materials over SiO . W = H = 40 nm and
G = 30 nm are kept constant. Resistance and reactance, respectively, for (a)-(b) Au, (c)-(d) Ag, (e)-(f) Cu, (g)-(h) Al and (i)-(j) PEC. Horizontal semi transparent
planes show zero crosses in reactance.
where
is the plasma wavelength, and both
and
coefficients determining the offset and slope of the linear relation.
correspond to the resonances of the ideal
The values for
non-dispersive PEC case given the same geometry. Apart from
the wavelength shift each material will give rise to different
) in the antenna, that can be qualiOhmic losses (
tatively classified according to the imaginary part of the permit. Although (1)
tivity as
serves as a good description of the wavelength scaling, a more
convenient form is given by (2), linearly relating both total anand the associated resonance with
tenna length
two parameters
(slope) and
(offset) that will depend in each case on the material and geometric properties of
the setup. This formula is easy to use for making a practical design
(2)
Fig. 6 consists of slices of Fig. 5 for specific configurations. As
discussed before, even if there is only one physical resonance,
resonant frequency can be defined in different ways:
1. at zero values of the reactance going from negative to positive (
);
DE ARQUER et al.: ENGINEERING THE INPUT IMPEDANCE OF OPTICAL NANO DIPOLE ANTENNAS
TABLE I
LINEAR FIT OF INPUT IMPEDANCE RESONANCE POSITIONS FOR SEVERAL
MATERIAL CONFIGURATIONS AS A FUNCTION OF L . W
H
AND
G = 30 nm
= = 40 nm
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40 nm
= 30 nm
= 110 nm
SiO
=2 +
= 30 nm
SiO
= 40 nm
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IEEE TRANSACTIONS ON ANTENNAS AND PROPAGATION, VOL. 59, NO. 9, SEPTEMBER 2011
=15
= 40 nm
= = 40 nm
=15
= = 40 nm
= 110 nm
TABLE II
LINEAR FIT OF EXTINCTION CROSS SECTION RESONANCE WAVELENGTHS FOR
PLANE WAVE ILLUMINATION AS A FUNCTION OF L . W
H
AND
G
. SUBSTRATE WITH REFRACTIVE INDEX n
:
= 30 nm
= = 40 nm
=15
but blue shifted with respect to gap feeding. A huge field enhancement appears now in the vicinity of the gap, where there
is no current flowing at all. Each nanorod indeed presents at
its ends zero current and a maximum value somewhere in the
middle, depending on the relative position and the strength of
the coupling [Fig. 8(g)(i)]. To overcome the mismatch introduced by the gap for the plane wave illumination in the currents
distribution, the use of one equivalent rod without gap was proposed in [21]. However, under this assumption the results are
red-shifted a lot, about 500 nm, compared to the same length
dipole with gap excitation. Resonances corresponding to the extinction peak values are analyzed for Au, Ag and PEC when
varying dipole arm length as it was done for the gap excita, subtion, this time with constant refractive index,
strate (Table II). The same shifts appear because of the material dispersive properties, but the resonant positions are overall
= 10 nm
= 1 nm
blue shifted compared with gap excitation. Differences are evident in the offset of the wavelength-dipole length relation, but
almost negligible for the slopes, where for two significant digits
the only difference appears for the PEC configuration. Far and
near field resonance shifts under plane wave illumination were
also reported in [41], [42] for single cylindrical nanorods but as
a function of their radii.
Now that the comparison of the two excitation methods has
been accomplished, a full analysis of the effect of the gap for
the plane wave excitation is performed. The gap size is crucial since it determines the coupling between the two dipole
arms, in this way affecting the far field response of the structure
and shifting the obtained resonances. Plasmon resonance spec) dependence on coupled nanorod antenna ditral position (
mensions has been studied extensively before [40][42]. However, little attention has been given to the spectral shape, i.e.,
the full width at half maximum (FWHM) of these resonances
[42]. This parameter is of great importance for several applications ranging from localized surface plasmon resonance (LSPR)
sensing to plasmonic lasing [43], where high quality resonators
having sharp lineshapes are required. For that reason, in addition
maps [Fig. 8(a) and (e)], for each
to the
and
set a full characterization of the normalized extinc(taken as the extinction cross section divided
tion spectra
by the antenna horizontal area) is given, by means of analyzing
, linewidth
, and
its peak
DE ARQUER et al.: ENGINEERING THE INPUT IMPEDANCE OF OPTICAL NANO DIPOLE ANTENNAS
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Fig. 9. The amplitude of the current distribution jJ j along the dipole integrated
over its cross section at resonance for Au over a n
: substrate with W
H
and L
for several gap sizes.
= 40 nm
= 110 nm
=15
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IEEE TRANSACTIONS ON ANTENNAS AND PROPAGATION, VOL. 59, NO. 9, SEPTEMBER 2011
losses due to dispersive not PEC materials, the remaining aspects of the behavior are similar to the behavior of classical antennas at microwave and RF frequencies. Transfer of know-how
from these areas is very feasible. A linear relation for the resonances in terms of the antenna length was introduced, as well as
some basic design rules. The effect of the dispersive properties
of some important metals was studied for the input impedance.
Resembling [21], a shift comparison
was observed for gap excitation. Gold produces the bigger
redshift, which is a good characteristic for designing subwavelength structures, but because of its permittivity, also presents
than silver and other metals. Copper
higher absorption and
shows a similar response than gold making both of them particularly suited for red and infrared wavelengths. Silver is less
redshifted but has certain practical issues related to oxidation.
Aluminium is the one closest to the ideal PEC case, although it
presents larger losses. Concerning losses, in the range 5001200
. Therefore, a trade-off among the desired working window, device size, and material characteristics
in each environment must be accomplished in the design and
engineering of the input impedance. The study of plane wave
excitation reveals that the phenomenology of this configuration
is not the same as for gap excitation, where the coupling between dipole arms is conductive instead of capacitive. This difference, in addition to the width influence on the far field, introduces a considerable blue shift in the cross section resonances.
A strong dependence of the scattering properties on antenna gap
and width values was shown under this illumination. The gap
influence on the extinction amplitude and peak position can be
understood in terms of input impedance as an increase and redshift in its values. It was shown that the antenna width is crucial
to accurately determine the values of the cross sections.
Further research, for example using different materials for
the individual nanorods could also introduce interesting properties in the frequency response of the system. Also, radiating
quantum dots can be studied. The intriguing world of nanocircuitry and the engineering of these devices represent an incredible challenge. It is shown that a proper design and the full understanding of each individual block and its connections undeniably requires a thorough study of the antenna input impedance.
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DE ARQUER et al.: ENGINEERING THE INPUT IMPEDANCE OF OPTICAL NANO DIPOLE ANTENNAS
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Victor Moshchalkov was born in Russia. He received the M.Sc., Ph.D., and Habilitation degrees
in physics from the Lomonosov Moscow State
University, Moscow, Russia, in 1975, 1978, and
1985, respectively.
From 1978 to 1988, he was a Research Physicist,
Assistant Professor, and Professor at the Lomonosov
Moscow State University where, in 1988, he became
Head of the Laboratory of High Temperature Superconductivity. Since 1986, he has held a number
of positions as Guest Scientist or Guest Professor
at Toronto University, Canada, TH Darmstadt, Marburg University, RWTH
Aachen, Germany, Centre dEtudes Nuclaires de Grenoble, France. In 1991,
he joined the Katholieke Universiteit Leuven, Leuven, Belgium, as a Visiting
Professor and where he became a Full Professor in 1993. He has over 780
publications in international peer reviewed journals and more than 9300
citations.
Prof. Moshchalkov has received several awards: the Young Researcher award
in 1986, the High Education Scientific Prize in 1988, the ISI Thomson Scientific Award Top Cited Paper in Flanders in 2000, the Dr. A.De LeeuwDamry-Bourlart Prize for Exact Sciences from the Flemish FWO in 2005, and
the Methusalem Research Award in 2009. He was a finalist for the EU Descartes
Research Prize in 2006. He is an American Physical Society Fellow since 2007.
He was the Chairman of the ESF Program Vortex Matter in Superconductors-VORTEX from 1999 until 2004. He became the Director of the INPAC
Institute for Nanoscale Physics and Chemistry (Center of Excellence at the K.U.
Leuven) in 2005. Since 2007, he is also the Chairman of the ESF-NES program,
which includes 60 teams from 15 European countries. He was an invited speaker
at 96 international conferences and workshops, and he is Founder of the new
series of International Conferences on Vortex Matter in Nanostructured Superconductors. He is a member of the International Advisory Committee of 34
international conferences. He has been, or is, Promoter of 48 Ph.D. theses (12
at the Moscow State University and 36 at the K.U. Leuven).