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The effects of material properties and tube array settings on gassolid ow and heat transfer characteristics in uidized beds with tubes are investigated by the combined approach of computational uid dynamics and discrete
element method, incorporated with heat transfer models. First, the effect of material properties is illustrated by
considering cohesive and non-cohesive powders with different particle sizes. The contributions of different heat
transfer mechanisms are discussed at two tube temperatures. Signicant differences of gassolid ow between
cohesive and non-cohesive powders are observed. The results reveal that conductive heat transfer between a
uidized bed and a tube is dominant for small cohesive particles while convective heat transfer is dominant
for large non-cohesive particles. Then, the uniformity of particle velocity and temperature elds is analyzed. It
is shown that material properties and gas velocity affect the uniformity of particle velocity and temperature in
a complicated manner. Finally, the effect of tube array settings is examined in terms of two geometrical parameters for both in-line and staggered settings. Complicated gassolid ow and heat transfer characteristics are
observed. An effort is made to link macroscopic observations to microscopic information such as local porosity
and contact number between uidized particles and tubes. The ndings should be helpful for the optimization
of operation and design of uidized systems with tubes.
2015 Elsevier B.V. All rights reserved.
1. Introduction
Fluidized bed reactors are widely used in industries mainly due to
their high heat and mass transfer capability. Immersed surfaces such
as vertical or horizontal tubes, ns, and water walls are usually adopted
to control ow and heat transfer. Heat transfer performance is affected
by many factors such as material properties of gas and solid phases,
geometrical settings and operating conditions. In the past, many macroscopic studies have been carried out in this eld, leading to the formulation of various correlations to determine the heat transfer coefcient
(HTC) of uidized beds as, for example, summarized by Kunii and
Levenspiel [1] and Molerus and Wirth [2]. These correlations have
shown their value in solving some practical problems. However, the
predictions by some correlations show signicant differences partly
due to negligence of certain parameters and unknown experimental
set-up and conditions [3]. To produce equations that can be generally
applied to different systems, microscopic understanding of ow
and heat transfer mechanisms at a particle scale is helpful. Such understanding can be obtained through experimental and/or numerical
Corresponding author at: Laboratory for Simulation and Modelling of Particulate
Systems, Department of Chemical Engineering, Monash University, Clayton, VIC 3800,
Australia. Tel: +61 3 99050845.
E-mail address: qinfu.hou@monash.edu (Q.F. Hou).
http://dx.doi.org/10.1016/j.powtec.2015.03.028
0032-5910/ 2015 Elsevier B.V. All rights reserved.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
approach [11,12,14]. The contributions of different heat transfer mechanisms are discussed [11], and the effects of some material properties
such as particle size and particle thermal conductivity are examined
[12,14]. In uidized beds, uniform particle velocity and temperature
distributions are often desired for heat transfer and chemical reactions.
If the uniformity is not good enough, hot spot, as pointed out by Kaneko
et al. [30], could be formed. Somehow, this important issue has not been
addressed in detail in the previous studies.
A tube array rather than a single tube is often used in uidization
systems. One major concern is the setting of a tube array, related to
heat transfer and tube erosion [3133]. Previous studies of such systems
have been mainly conducted by using two-uid models [3436] or
by experimental approaches [3739]. Recent studies on the setting
of a tube array are carried out by means of the CFDDEM approach
[40,41]. Some interesting ndings are presented, but controversies can
also be identied. For example, the signicant effect of tube pitch on
the erosion has been demonstrated [35]. While no signicant difference
in terms of bubbling behaviors or heat transfer between different tube
settings (in-line and staggered) is observed [34,41], quite different
factors underlying heat transfer such as particle impacts and bubble behaviors are predicted by the CFDDEM approach [40]. A possible reason
could be that particle scale interactions are not sufciently considered.
The different observations indicate that there is a need for further investigation of the effect of tube array settings on gassolid ow behavior. In
particular, the effect on heat transfer and the underlying mechanisms
should be properly understood.
In this work, in connection with our previous efforts [14,15], two
signicant concerns relevant to gassolid ows and heat transfer characteristics are addressed by using the combined CFDDEM approach. Firstly,
the effect of material properties for different types of particles including
non-cohesive and cohesive particles is investigated for a uidized bed
with a horizontal tube. The uniformity of velocity and temperature elds
is quantied. Secondly, the effect of tube array settings is investigated for
a uidized bed with multiple horizontal tubes. The complicated variation
of heat ux between the uidized bed and tubes is discussed in terms of
microscopic information such as local porosity and contact number between particles and tubes. The ndings should be useful for better understanding and prediction of heat transfer in gas uidization.
2. Model description
2.1. Governing equations for solid phase
Here, gas uidization is considered to be composed of a discrete solid
phase and a continuum gas phase. The solid phase is described by DEM,
originally proposed by Cundall and Strack [42]. At any given time t, the
equations governing the translational and rotational motions of particle
i can be written as:
mi dvi =dt j f e;ij f d;ij f v;ij f pf ;i mi g;
and
Ii di =dt j Tt;ij Tr;ij ;
where the equation for the van der Waals force is written as:
f v;ij
3 3
64Ri Rj h Ri Rj
2 n:
2
h2 2Ri h 2Rj h 4Ri Rj
h2 2Ri h 2Rj h
Ha
6
The forces involved are: particleuid interaction force fpf,i, the gravitational force mig and the forces between particles (and between particles and walls) which include the elastic force fe,ij, the viscous damping
force fd,ij and the cohesive force fv,ij. Note that the cohesive force fv,ij,
considered here is the van der Waals force given by Eq. (3), which depends on the Hamaker constant Ha and the separation h of the interacting
surfaces along the line joining the centers of particles i and j. Ri and Rj are
the radii of particles i and j respectively. A minimum separation hmin is
used in the calculation of fv,ij to represent the physical repulsive nature
and avoid the singular attractive force when h = 0. This treatment has
been proved to be valid for particles down to 1 m [4345]. The torque
acting on particle i due to particle j includes two components: Tt,ij
which is generated by the tangential force and causes particle i to rotate,
and Tr,ij which, commonly known as the rolling friction torque, is generated by asymmetric normal contact forces and slows down the relative
rotation between contacting particles [46,47]. If particle i undergoes multiple interactions, the individual interaction forces and torques are
summed up for all particles interacting with particle i. The equations
used to calculate the particleparticle interaction forces and torques,
and particleuid interaction forces have been well established as, for example, reviewed by Zhu et al. [48]. The equations used for the present
work are the same as those used in our previous studies [20,49].
The heat transfer between particle i and its surroundings have three
modes: convection with uid, conduction with other particles, tubes or
walls, and radiation with its local environment. According to the energy
balance, the governing equation for particle i can be written as [10]:
its local surrounding uid; Q i;rad is the radiative heat exchange rate
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
Table 1
Equations to calculate heat exchange rates.
Heat exchange rates
Convective
Equation
Q f ;wall 0:037Re0:8 Pr
Conductive
Radiative
(a)
(b)
1=3
k f Aw T=L
q
q 1
rsf
Q i;j T j T i r 2r
R2i r 2 r R2i H
r ij 1=kpi 1=kpj 2 R2i H R2i r 2
dr
kf
sij
1=2
= pi cpi k
pj cpj kpj
Q i;j c T j T i r 2c t c
k
T j ji=k
Q i;rad eAi T 4local;i T 4i ; Q f ;rad ef Af T 4local;i T 4f where T local;i f T f ; 1f j1
(c)
and Te in the vicinity of the tube are obtained for an annular region
around the tube with a thickness of 5dp in its radial direction. All these
treatments have been used in our previous study and proved to work
satisfactorily [14].
2.2. Governing equations for uid phase
The uid phase, air to be specic for this study, is treated as a continuum phase and modeled in a way similar to the one widely used in the
conventional two-uid model [51]. In this connection, there are three
sets of governing equations, developed by Anderson and Jackson [51].
Different governing equations may lead to different results, depending
on the systems considered. According to Zhou et al. [20], Set II and in
particular Set I can be used generally, and Set III can only be used conditionally. In this work, Set I is used. Thus, the conservations of mass and
momentum in terms of the local averaged variables over a computational cell are given by:
.
f f
t f f u 0;
and
.
f f u t f f uu pFf p f f g:
(d)
(e)
(f)
where u, f, p and Ffp are the uid velocity, density, pressure and volumetric
h
i
1
Table 2
Physical and geometrical parameters used in the simulations.a
Variables
Values
100 1280
Z = 50
50 640
22
30,000
40
0.1
1440
1.1
380
840.0
24.4
200
0.3
0.01
0.8
1 107
0.3
2.10 1021
PM/(RTf)
1.511 106Tf3/2/(Tf + 120.0)
2.873 103 + 7.760 105 Tf
1002.737 + 1.232 102 Tf
These are for the base case. Some parameters may vary in different cases, as specied
in the text or gure caption.
kv
Q f ;i Q f ;wall Q f ;tube Q f ;rad =V , where Q f ;i is the conQ i1
the convective heat exchange rate between uid and tubes; Q f ;wall
is the convective heat exchange rate between uid and a wall; and
Q f ;rad is the radiative heat exchange rate between uid and its environment. In the present work, because of the low emissivity of
uid, the radiative heat transfer between uid and its environment
is ignored for simplicity.
2.3. CFDDEM coupling scheme
The methods of numerical solutions to problems requiring CFD
DEM coupling have been well established [19,20,54]. Heat transfer
models have also been incorporated into this approach as demonstrated
Table 3
Properties of three powders.
Parameter
dp, mm
H a, J
umf, m/s
0.1
0.1
0.5
2.10 1021
0
2.10 1021
0.0072
0.0072
0.15
Powder
A
A0
B
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
Fig. 1. Selection of unit cells for different settings: (a) square and (b) triangular.
t=0s
(a)
2s
6s
2s
(b)
The number of particles is constant for all the cases in this work. It
should be noted that the van der Waals force is the only considered cohesive force. In principle, the Hamaker constant depends on many variables related to physical and chemical properties, such as the surface
roughness or asperity, medium chemistry. In the present study the
Hamaker constant of 2.10 1021 is adopted, which has been used in
our previous study to reasonably reproduce the behaviors of cohesive
particles [49]. Walls are assumed to have the same material properties
as the particles for convenience. Spherical particles at a temperature of
25 C are used as the initial solid phase uidized in a container with a
thickness of four particle diameter (dp). The periodic boundary condition is applied to the front and rear directions to eliminate the effect
of walls. To remove the effect of the side walls, the selected bed widths
should be sufcient as the side wall can only affect the ow up to 10dp
even in a rather dense particulate ow (see, for example, [55]). For
the above geometry, two-dimensional CFD and three-dimensional
DEM are used as done by Feng et al. [54]. This treatment should be reasonable, given that the bed width (100dp) is much larger than its thickness (4dp) and the tubes are set horizontally. For the CFD computation
6s
2s
6s
(c)
Fig. 2. Gassolid ow pattern in uidized beds for different powders when uf/umf = 5 and tube temperature Ts = 200 C: (a) Powder A, (b) Powder A0, and (c) Powder B. All particles are
shown, colored by their coordination number (CN). (For interpretation of the references to color in this gure legend, the reader is referred to the web version of this article.)
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
Convection
Conduction
Powder A
0.1
0.0
0.2
0.2
Convection
Conduction
Powder A0
0.1
0.0
2.5 Powder B
2.0
1.5
1.0
0.5
0.0
2.0
Convection
Conduction
2.5
3.0
3.5
4.0
Time (s)
(a)
100
80
Powder A
Powder A0
Powder B
60
40
20
0
100
80
60
Powder A
Powder A0
Powder B
40
20
0
2.0
2.5
3.0
3.5
4.0
Time (s)
(b)
Fig. 3. Heat exchange rates between the uidized bed and the tube (a), and their percentage contributions to the total heat exchange for different powders (b).
two major treatments are adopted for the transfer of information between 2D CFD and 3D DEM. The rst treatment is used to obtain the
local porosities with only one control volume assumed in the thickness
direction. The particles in a given CFD cell are determined only by the
coordinates in the x and z directions. The second treatment is used for
the transfer of momentum and energy sources assuming that the
sources in the bed thickness direction are negligible. The non-slip
boundary condition is applied to the walls, and zero diffusion ux
condition to the outlet for ow and heat transfer.
To investigate the effect of tube array settings, particle diameter dp is
set to 0.6 mm with a numerically determined minimum uidization velocity (umf) of 0.36 m/s. The bed of 105 particles has a width of 160dp and
a height of 1,000dp. Tube diameter is 20dp. As the main aim of this part is
to examine the effect of tube array settings, all the cases are carried out
at a low tube temperature (Ts) of 200 C where radiative heat transfer is
negligible [14]. The inlet gas velocity is set to 3umf. Two types of tube
array settings are considered as shown in Fig. 1. One setting is square
(in-line) and the other is triangular (staggered). Two unit cells are chosen accordingly for analysis as shown in Fig. 1. It should be noted that
this treatment is reasonable, as shown in the present study that the interaction between neighboring tubes is insignicant if pitch length is
larger than 2.5D (here, D is tube diameter). The relative tube position
is quantied by two parameters: one is angle between the line joining
the centers of the tubes and the horizontal line in the cross-section of
the tubes, and the other is pitch length L. Angles of 30, 45 and 60 and
center-to-center pitch lengths in the range of 1.54D are adopted for
triangular settings.
0.2
(a)
0.1
Porosity (-)
1.0
0.8
0.6
Powder A
Powder A0
Powder B
100
0.0
0.03
0.02
0.01
0.00
0.010
(b)
(c)
0.005
0.000
(d)
0.010
0.005
50
0.000
2.0
0
3.0
2.5
3.0
3.5
4.0
Time (s)
3.2
3.4
3.6
3.8
4.0
Time (s)
Fig. 4. Evolution of the local porosity and the contact number between particles and the
tube for different powders.
Fig. 5. Evolution of heat exchange rates by different conductive heat transfer mechanisms:
(a) particleuidtube under non-contact condition, (b) particleuidtube under
contact condition, (c) particletube with collisional contacts, and (d) particletube with
static (enduring) contacts.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
Table 4
Time-averaged percentage contributions of different heat transfer mechanisms.
Conditions
5 umf
Mechanisms
A0
A0
Conduction
Convection
Particleuidtube non-contact
Particleuidtube contact
Particletube collisional contact
Particletube static contact
94.4%
5.6%
91.7%
5.7%
0.5%
2.1%
94.2%
5.8%
91.7%
5.7%
0.5%
2.1%
20.1%
79.9%
91.7%
5.7%
0.5%
2.1%
83.4%
16.6%
93.6%
5.0%
0.3%
1.1%
83.2%
16.8%
93.7%
4.9%
0.3%
1.1%
8.7%
91.3%
91.8%
7.7%
0.3%
0.2%
10 umf
t=0.02s
t=1s
t=2s
interaction force varies with particle size, and hence, different particleparticle contact conditions are generated [49]. It can also be
reected in particle coordination number (CN) and different sizes of
bubbles or large voids within the bubbling uidized beds at the same
ratio of uf/umf. These differences can generate different heat transfer
characteristics as observed in the cases of uidized beds without tubes
[15].
The tube exchanges heat with its surroundings mainly through
conduction with particles and convection to the gas ow at low temperatures [14,57]. Heat exchange rates through the two modes are uctuating temporally for different powders, as shown in Fig. 3(a). For Powders
A and A0, conductive heat transfer between the uidized bed and
the tube is dominant. But for Powder B, convective heat transfer is
dominant. These can be clearly observed in terms of the percentage contribution of heat exchange rates, as given in Fig. 3(b). For small particles,
the van der Waals force at the given Hamaker constant affects heat
transfer slightly. Only minor differences can be observed between Powders A and A0 in terms of the contributions of different heat transfer
modes. This is clearly shown in Table 5 in Section 4.2 from the timeaveraged percentage contributions of different heat transfer modes. It
should be noted that if the Hamaker constant is large enough, different
heat transfer characteristics can be observed as demonstrated in our
previous study [15].
These observations are related to the local porosity and the contacts
between particles and the tube. As shown in Fig. 4, the local porosity
around the tube for different powders has only minor differences except
that large uctuations are observed for Powder B. This also applies to
the contact number between particles and the tube. Smaller particles
t=3s
t=4s
t=5s
t=6s
Fig. 6. Solid ow pattern for Powder A when Ts = 600 C. All particles are shown, colored by their temperatures. (For interpretation of the references to color in this gure legend, the
reader is referred to the web version of this article.)
0.4
100
0.2
60
40
20
0.0
3.0
(a)
Conduction
Convection
Radiation
80
Percentage (%)
Conduction
Convection
Radiation
3.2
3.4
3.6
Time (s)
3.8
4.0
3.0
(b)
3.2
3.4
3.6
3.8
4.0
Time (s)
Fig. 7. Evolution of heat exchange rates and their percentage contributions at Ts = 600 C.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
5 umf
Mechanisms
A0
A0
Conduction
Convection
Radiation
41.9%
3.8%
54.3%
44.0%
3.5%
52.5%
10.5%
46.0%
43.5%
32.0%
5.7%
62.3%
32.7%
5.5%
61.8%
5.0%
51.7%
43.3%
10 umf
can enhance conductive heat transfer between the tube and the uidized bed due to their relatively larger total contact area at a given porosity [15]. The differences in ow behavior and contact conditions will
result in different heat transfer behaviors, as discussed in the following
sub-sections.
Conductive heat transfer between the tube and the uidized bed is
dominant for the small particles. The contributions of four different conductive heat transfer mechanisms to the total conductive heat transfer
are examined here. The evolution of different conductive heat exchange
rates is shown in Fig. 5. It can be observed that the heat transfer through
the tubeuidparticle path under non-contact condition is the largest
one. The second largest is the heat transfer through the path of tube
uidparticle under contact condition. These results are consistent
with those reported in the literature, where gas lm around the tube
plays an important role in heat transfer between an immersed surface
and a uidized bed [1]. Due to the short contact time and small solid
contact area, the conductive heat exchange rates through the particle
tube path are small. The contact time could vary with the velocities of
colliding particles and the gassolid ow. For an approximation of impact contact duration tc, Eq. (8) can be used, where m is the equivalent
t=0.1s
1s
The contributions of different mechanisms vary for different powders as listed in Table 4. The contribution of each conductive heat transfer mechanism to the total conductive heat transfer is also quantied
(here 41xi = 100 % where xi is the contribution of conductive heat
transfer by mechanism i). For Powders A and A0, the conductive heat
transfer is dominant with its percentages around 90%. For Powder B,
the convective heat transfer is dominant with its percentage around
80%. With the increase of gas velocity, the contribution of convective
heat transfer increases and that of conductive heat transfer reduces.
One reason for this observation is the enhanced dilute gassolid ow
due to the increase of gas velocity. Although different powders have
different dominant heat transfer modes, the results indicate that heat
transfer through the particleuidtube path is dominant for conduction in all the cases studied. The contribution of heat exchange rate
through the particleuidtube path increases with the increase of
gas velocity while that through the particletube path decreases.
Heat transfer between a tube and a uidized bed by radiation becomes important at high temperatures [14,57]. The proposed model
can account for this factor. As an example, this work also investigates
the heat transfer at a high tube temperature (Ts) of 600 C for different
powders. As shown in Fig. 6, particles near the tube are rst heated, and
then these hot particles move into other parts of the bed, exchanging
heat with other cold particles. In this process, particle temperature
5s
6s
(a)
DoV
(b)
Fig. 8. Deviation of velocity (DoV) of all particles in uidized beds during heating process by a tube at Ts = 600 C and uf/umf = 10: (a) Powder A and (b) Powder B.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
t=0.1s
1s
5s
6s
(a)
DoT
(b)
Fig. 9. Deviation of temperature (DoT) of all particles in uidized beds during heating process by a tube at Ts = 600 C and uf/umf = 10: (a) Powder A and (b) Powder B.
1.0
1.0
0.8
0.8
0.6
0.4
0.1
0.0
(a)
0.6
0.4
0.2
DoT (-)
DoT (-)
0.2
2.82
DoV (-)
DoV (-)
distribution is not uniform, and areas with relatively high or low temperatures are observed.
The evolution of heat exchange rates at a high temperature and their
contributions are demonstrated in Fig. 7 for Ts = 600 C. At this temperature, the conductive heat exchange rate is the largest, the convective
one is the smallest, and the radiative one has an intermediate value
varying steadily. The conductive heat exchange rate uctuates with
values smaller than that of radiative heat transfer at some instants.
Their contributions to the total heat exchange rate by all heat transfer
modes are analyzed as shown in Fig. 7(b). The percentage contributions
uctuate and the radiative heat transfer has the largest value. Their contributions are compared quantitatively in terms of time-averaged values
in Table 5 for different powders and gas velocities at Ts = 600 C. It indicates that the radiative heat transfer is an important mode in all the
cases studied. For small particles, the contribution of radiation is larger
than that of conduction which is dominant at low temperatures. However, for large particles, the convective heat transfer is still dominant
2
Time (s)
0.1
0.0
(b)
2
Time (s)
Fig. 10. Evolution of bed averaged DoV and DoT of individual particles: (a) Powder A and (b) Powder B.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
5 umf
Index
A0
A0
0.129
0.129
0.033
0.006
0.126
0.125
0.031
0.006
0.232
0.235
0.016
2.86E4
0.125
0.127
0.019
1.74E3
0.121
0.127
0.022
2.01E3
0.239
0.245
8.49E3
1.10E4
Ts = 200 C
Ts = 600 C
Ts = 200 C
Ts = 600 C
DoV
DoV
DoT
DoT
10 umf
for individual particles, dened as |1 ui/bui N | where ui is the magnitude of particle velocity and b N is the average over all particles. The
other parameter is the deviation of temperature (DoT) from the mean
temperature, dened as |1 Ti/b Ti N |.
Heat transfer characteristics and the uniformity of particle temperature are closely related to the motion of particles. The deviation from the
mean velocity of individual particles is shown in Fig. 8 for Powders A
and B. The particles in the vicinity of the tube have large DoVs because
of the disturbance induced by the tube. The deviation diminishes in
other areas as a result of the momentum exchange between particles.
Large DoVs of small particles are often observed in the middle of the uidized bed; conversely, DoVs are large near the walls for large particles.
The deviation from the mean temperature of individual particles is
shown in Fig. 9 for Powders A and B, under the conditions corresponding to those of Fig. 8. Compared to DoV, DoT is rather small as a result
of high heat transfer capability of uidized beds. However, a spatial
distribution of DoT can still be observed. A large DoT occurs in the
vicinity of the tube due to heat exchange between the bed and the
tube. This indicates the possibility of observing hot spots with nonuniform particle temperatures in the bed.
To quantify the uniformity of particle velocities and temperatures at
a bed scale, the bed averaged DoV and DoT of individual particles
are shown in Fig. 10 for Powders A and B. It can be seen that the bed
averaged DoV decreases rather quickly to a small value while the bed
averaged DoT takes a longer time. The values vary for different powders.
To show the effect of material properties on DoV and DoT, the timeaveraged values are listed in Table 6. The time-average is carried out
within a xed time frame (06 s) in which period DoV and DoT decrease
to rather small values. It is found that a time-average with a longer time
will give a smaller value because the negligible small values after 6 s are
t=0 s
t=0.4 s
t=0.8 s
t=1.6 s
t=6.0 s
(a)
(b)
Fig. 11. Gassolid ow patterns in uidized beds with a tube array: (a) for different times when = 45 and (b) for different settings when t = 6.0 s. The settings include a square one
( = 0) and three triangular ones ( = 30, 45, and 60) from the left to right. All particles in each case are shown.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
10
1.0
2.0
#1
Tube #1
Tube #2
#2
1.5
1.0
0.5
0.0
2.0
2.5
3.0
(a)
3.5
(b)
100
0.6
0.4
0.2
2.5
3.0
3.5
4.0
Time (s)
Tube #1
Tube #2
80
Percentage (%)
0.8
0.0
2.0
4.0
Time (s)
Tube #1
Tube #2
60
40
20
0
2.0
2.5
3.0
(c)
3.5
4.0
Time (s)
Fig. 12. Evolution of heat exchange rates for two representative tubes in a uidized bed: (a) total heat exchange rate, (b) conductive heat exchange rate, and (c) percentage of conductive
heat exchange rate to the total. The positions of two representative tubes (#1 and #2) are illustrated in the inset in (a). The square setting for this case has a pitch length of 1.5D.
1.0
Tube #1
Tube #2
0.9
75
100
50
25
0.8
0.7
0.6
Tube #1
Tube #2
0.5
0
(a)
2.0
2.5
3.0
Time (s)
3.5
4.0
0.4
2.0
(b)
2.5
3.0
3.5
4.0
Time (s)
Fig. 13. Evolution of: (a) the contact numbers between two representative tubes and uidized particles and (b) local porosity. The square setting for this case has a pitch length of 1.5D.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
11
Fig. 14. Heat exchange rates as a function of pitch length and angle: (a) convection, (b) conduction, and (c) total.
from a previous study [31]. The reason could be that if the pitch length is
larger than 2.5D, the effect of neighboring tubes becomes insignicant,
and hence the heat transfer between the uidized bed and the tube
considered is mainly determined by the surrounding gassolid ow
and takes place without much variation.
Heat exchange rates vary with angle in a complicated manner at
different pitch lengths as shown in Fig. 14. Generally, total heat
exchange rate decreases with the increase of . The convective heat
exchange rate shows a similar trend to that of the total heat exchange
rate. The conductive heat exchange rate varies complicatedly for
different pitch lengths, as discussed below. It can be seen that the conductive heat exchange rate plays a role as important as the convective
heat exchange rate for the system considered.
Heat exchange rates vary differently with in a certain range of
pitch lengths. For convenience, the pitch length is classied into three
categories according to the variation of conductive heat exchange
rate: small (1.5 and 2D), intermediate (2.5 and 3D), and large (3.5 and
4D). For the small pitch range, the conductive heat exchange rate
Fig. 15. Contact number (a) and local porosity (b) as a function of pitch length and angle.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
12
increases rst, and then decreases with the increase of . The turning
points vary with the pitch length. The convective heat exchange rate reduces consistently with the increase of . As the sum of conductive and
convective heat exchange rates, the total heat exchange rate decreases
consistently for a pitch length of 1.5D or increases a little rst and
then decreases for a pitch length of 2D with the increase of . For the intermediate range, the convective heat exchange rate decreases consistently while the conductive heat exchange rate decreases rst and
then increases slightly with the increase of . The total heat exchange
rate decreases rst and then becomes constant for a pitch length of
2.5D, or decreases consistently for a pitch length of 3D. In the large
pitch range, variations in all heat exchange rates are insignicant.
The change of heat exchange rates can be understood from the
microscopic information such as contact number and local porosity.
Contact numbers under various conditions are shown in Fig. 15(a),
indicating consistent variations with the change of conductive heat
exchange rate shown in Fig. 14(b). Conductive heat transfer occurs
when particles are in direct contact with or close enough to a given
tube according to the heat transfer mechanisms discussed. Hence, as
expected, a connection between conductive heat exchange rate and
contact number is observed, although other factors such as colliding velocity and contact time could affect the conductive heat transfer. Based
on the predictions, contact number can be considered as a main index
determining the conductive heat exchange rate for the system investigated. The time-averaged local porosity (Fig. 15(b)) is closely related
to the convective heat transfer. However, only small change is observed
at a given inlet gas velocity, which is consistent with the variation of
corresponding convective heat exchange rate. Such information may
be helpful for the design and optimization of tube arrays for heat
transfer in uidized beds.
5. Conclusions
The combined CFDDEM approach with heat transfer models incorporated is used to investigate the effects of material properties and
geometrical settings on gassolid ow and heat transfer characteristics
in uidized beds with tubes. The following conclusions can be drawn
from the present study:
The convective heat transfer is dominant for large, non-cohesive
particles while the conductive heat transfer is dominant for small, cohesive particles at low temperatures, when the radiative heat transfer
is negligible. Heat exchange rate through the particleuidtube path
under non-contact condition is dominant of the conductive heat
transfer mode. Radiative heat transfer becomes important at high
temperatures (higher than ~ 600 C). Radiative heat transfer can be
dominant for small particles under certain conditions.
The effect of material properties on the uniformity of particle velocities
and temperatures is signicant. Large particles have a low uniformity
of particle velocities but high uniformity of particle temperatures. For
a given Hamaker constant, the cohesive force affects both the velocity
and temperature elds insignicantly. Material properties and operating conditions should be selected carefully by considering the uniformity of particle velocities and temperature elds.
The effect of gas velocity on the uniformity of particle velocities and
temperatures is complicated. On one hand, gas velocity has little effect
on the uniformity of particle velocities. On the other hand, a large gas
velocity can improve the uniformity of particle temperatures. A high
tube temperature can also result in a high uniformity of particle
temperatures.
The effect of tube array setting is complicated as reected in the changes in the gassolid ow characteristics and heat exchange rates. It can
be related to microscopic information such as the local porosity, and
contact number between particles and a given tube. Conductive heat
exchange rate is closely related to the contact number while convective
rate is closely related to the local porosity.
Acknowledgments
The authors are grateful to the Australian Research Council
(FF0883231) for the nancial support. This work was supported by an
award under the Merit Allocation Scheme on the NCI National Facility
at the ANU.
References
[1] D. Kunii, O. Levenspiel, Fluidization Engineering, Butterworth-Heinemann, Boston,
1991.
[2] O. Molerus, K.E. Wirth, Heat Transfer in Fluidized Beds, Chapman and Hall, London,
1997.
[3] S.N. Oka, Fluidized Bed Combustion, Marcel Dekker, Inc., New York, 2003.
[4] A.P. Collier, A.N. Hayhurst, J.L. Richardson, S.A. Scott, The heat transfer coefcient
between a particle and a bed (packed or uidised) of much larger particles, Chem.
Eng. Sci. 59 (2004) 46134620.
[5] M.S. Parmar, A.N. Hayhurst, The heat transfer coefcient for a freely moving sphere
in a bubbling uidised bed, Chem. Eng. Sci. 57 (2002) 34853494.
[6] S.A. Scott, J.F. Davidson, J.S. Dennis, A.N. Hayhurst, Heat transfer to a single sphere
immersed in beds of particles supplied by gas at rates above and below minimum
uidization, Ind. Eng. Chem. Res. 43 (2004) 56325644.
[7] K.F. Malone, B.H. Xu, Particle-scale simulation of heat transfer in liquid-uidised
beds, Powder Technol. 184 (2008) 189204.
[8] Y. Geng, D. Che, An extended DEMCFD model for char combustion in a bubbling
uidized bed combustor of inert sand, Chem. Eng. Sci. 66 (2011) 207219.
[9] H.S. Zhou, G. Flamant, D. Gauthier, Y. Flitris, Simulation of coal combustion in a bubbling uidized bed by distinct element method, Chem. Eng. Res. Des. 81 (2003)
11441149.
[10] Z.Y. Zhou, A.B. Yu, P. Zulli, Particle scale study of heat transfer in packed and bubbling uidized beds, AIChE J. 55 (2009) 868884.
[11] F.P. Di Maio, A. Di Renzo, D. Trevisan, Comparison of heat transfer models in DEM
CFD simulations of uidized beds with an immersed probe, Powder Technol. 193
(2009) 257265.
[12] Y.Z. Zhao, M.Q. Jiang, Y.L. Liu, J.Y. Zheng, Particle-scale simulation of the ow and
heat transfer behaviors in uidized bed with immersed tube, AIChE J. 55 (2009)
31093124.
[13] Z.Y. Zhou, A.B. Yu, P. Zulli, A new computational method for studying heat transfer in
uid bed reactors, Powder Technol. 197 (2010) 102110.
[14] Q.F. Hou, Z.Y. Zhou, A.B. Yu, Computational study of the heat transfer in bubbling
uidized beds with a horizontal tube, AIChE J. 58 (2012) 14221434.
[15] Q.F. Hou, Z.Y. Zhou, A.B. Yu, Computational study of the effects of material properties
on heat transfer in gas uidization, Ind. Eng. Chem. Res. 51 (2012) 1157211586.
[16] S.L. Yang, K. Luo, M.M. Fang, J.R. Fan, K.F. Cen, Discrete element study of solid mixing
behavior with temperature difference in three-dimensional bubbling uidized bed,
Ind. Eng. Chem. Res. 53 (2014) 70437055.
[17] Q.F. Hou, Z.Y. Zhou, A.B. Yu, Computational study of heat transfer in gas uidization,
Powders and Grains 2013: Proceedings of the 7th International Conference on
Micromechanics of Granular Media, 1542 2013, pp. 11141117.
[18] Z.Y. Zhou, Q.F. Hou, A.B. Yu, Particle scale simulation of heat transfer in uid bed reactors, in: A. Belmiloudi (Ed.), Heat Transfer Mathematical Modelling, Numerical
Methods and Information Technology, InTech 2011, pp. 383408.
[19] B.H. Xu, A.B. Yu, Numerical simulation of the gassolid ow in a uidized bed by
combining discrete particle method with computational uid dynamics, Chem.
Eng. Sci. 52 (1997) 27852809.
[20] Z.Y. Zhou, S.B. Kuang, K.W. Chu, A.B. Yu, Discrete particle simulation of particleuid
ow: model formulations and their applicability, J. Fluid Mech. 661 (2010) 482510.
[21] Y. Tsuji, T. Kawaguchi, T. Tanaka, Discrete particle simulation of two-dimensional
uidized bed, Powder Technol. 77 (1993) 7987.
[22] D. Geldart, Types of gas uidization, Powder Technol. 7 (1973) 285292.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028
13
[41] H. Wahyudi, K.W. Chu, A.B. Yu, Discrete particle simulation of heat transfer in
pressurized uidized bed with immersed cylinders, Powders and Grains 2013: Proceedings of the 7th International Conference on Micromechanics of Granular Media,
1542 2013, pp. 11181121.
[42] P.A. Cundall, O.D.L. Strack, A discrete numerical model for granular assemblies,
Geotechnique 29 (1979) 4765.
[43] R.Y. Yang, R.P. Zou, A.B. Yu, Computer simulation of the packing of ne particles,
Phys. Rev. E 62 (2000) 39003908.
[44] K.J. Dong, R.Y. Yang, R.P. Zou, A.B. Yu, Role of interparticle forces in the formation of
random loose packing, Phys. Rev. Lett. 96 (2006) 145505.
[45] K.J. Dong, R.Y. Yang, R.P. Zou, A.B. Yu, Settling of particles in liquids: effects of
material properties, AIChE J. 58 (2012) 14091421.
[46] Y.C. Zhou, B.D. Wright, R.Y. Yang, B.H. Xu, A.B. Yu, Rolling friction in the dynamic
simulation of sandpile formation, Physica A 269 (1999) 536553.
[47] Q.J. Zheng, H.P. Zhu, A.B. Yu, Finite element analysis of the rolling friction of a viscous
particle on a rigid plane, Powder Technol. 207 (2011) 401406.
[48] H.P. Zhu, Z.Y. Zhou, R.Y. Yang, A.B. Yu, Discrete particle simulation of particulate
systems: theoretical developments, Chem. Eng. Sci. 62 (2007) 33783396.
[49] Q.F. Hou, Z.Y. Zhou, A.B. Yu, Micromechanical modeling and analysis of different
ow regimes in gas uidization, Chem. Eng. Sci. 84 (2012) 449468.
[50] F.P. Incropera, D.P. Dewitt, Fundamentals of Heat and Mass Transfer, Fifth ed. John
Wiley & Sons, New York, 2002.
[51] T.B. Anderson, R. Jackson, Fluid mechanical description of uidized bedsequations
of motion, Ind. Eng. Chem. Fundam. 6 (1967) 527539.
[52] B.E. Launder, D.B. Spalding, The numerical computation of turbulent ows, Comput.
Methods Appl. Mech. Eng. 3 (1974) 269289.
[53] S.B. Kuang, A.B. Yu, Micromechanic modelling and analysis of the ow regimes in
horizontal pneumatic conveying, AIChE J. 57 (2011) 27082725.
[54] Y.Q. Feng, B.H. Xu, S.J. Zhang, A.B. Yu, P. Zulli, Discrete particle simulation of gas
uidization of particle mixtures, AIChE J. 50 (2004) 17131728.
[55] R.P. Zou, A.B. Yu, The packing of spheres in a cylindrical container: the thickness
effect, Chem. Eng. Sci. 50 (1995) 15041507.
[56] J. Schafer, S. Dippel, D.E. Wolf, Force schemes in simulations of granular materials, J.
Phys. I 6 (1996) 520.
[57] J.C. Chen, J.R. Grace, M.R. Golriz, Heat transfer in uidized beds: design methods,
Powder Technol. 150 (2005) 123132.
[58] J. Sun, M.M. Chen, A theoretical analysis of heat transfer due to particle impact, Int. J.
Heat Mass Transf. 31 (1988) 969975.
[59] Y.S. Wong, J.P.K. Seville, Single-particle motion and heat transfer in uidized beds,
AIChE J. 52 (2006) 40994109.
Please cite this article as: Q.F. Hou, et al., Gassolid ow and heat transfer in uidized beds with tubes: Effects of material properties and tube array
settings, Powder Technol. (2015), http://dx.doi.org/10.1016/j.powtec.2015.03.028