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A dual band terahertz metamaterial absorber

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2010 J. Phys. D: Appl. Phys. 43 225102

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IOP PUBLISHING JOURNAL OF PHYSICS D: APPLIED PHYSICS
J. Phys. D: Appl. Phys. 43 (2010) 225102 (5pp) doi:10.1088/0022-3727/43/22/225102

A dual band terahertz metamaterial


absorber
Hu Tao1 , C M Bingham2 , D Pilon3 , Kebin Fan1 , A C Strikwerda3 ,
D Shrekenhamer2 , W J Padilla2 , Xin Zhang1 and R D Averitt3
1
Department of Mechanical Engineering, Boston University, Boston, MA 02215, USA
2
Department of Physics, Boston College, Chestnut Hill, MA 02467, USA
3
Department of Physics, Boston University, Boston, MA 02215, USA
E-mail: xinz@bu.edu and raveritt@physics.bu.edu

Received 29 July 2009


Published 19 May 2010
Online at stacks.iop.org/JPhysD/43/225102

Abstract
We present the design, fabrication and characterization of a dual band metamaterial absorber
which experimentally shows two distinct absorption peaks of 0.85 at 1.4 THz and 0.94 at
3.0 THz. The dual band absorber consists of a dual band electric-field-coupled (ELC) resonator
and a metallic ground plane, separated by an 8 m dielectric spacer. Fine tuning of the two
absorption resonances is achieved by individually adjusting each ELC resonator geometry.
(Some figures in this article are in colour only in the electronic version)

Metamaterials consisting of artificially constructed electro- surface [12]. However, researchers have found that such ELC
magnetic (EM) materials have recently attracted considerable resonators could show similar resonance responses with the
interest due to their ability to exhibit engineered exotic EM EM wave propagating normal to the substrate and the electric
responses not available in nature, including negative refractive field aligned perpendicular to the resonators gap [10]. To
index, superlensing and cloaking [14]. Many of these ideas date, due to the limitations of currently available fabrication
were initially implemented at microwave frequencies due to the and characterization techniques, most terahertz metamaterials
simplicity in fabrication. Nevertheless, there has been substan- were made by patterning periodic SRRs in a single planar
tial progress and successful demonstrations of metamaterials form to show effective negative electric permittivity () or
extending from the terahertz through the visible frequencies negative magnetic permeability (). Additional layers or more
using micro/nano fabrication technologies during the past sev- complex structures need to be introduced for tailoring both
eral years [57]. Development of metamaterials at terahertz and , which is important to realize negative refractive index.
frequencies is especially important and attractive since there Tailoring the effective and also provides the means to
is a strong need to create components to realize applications engineer the impedance.
ranging from spectroscopic identification of hazardous materi- Recently, a narrow band microwave resonant metamaterial
als to noninvasive imaging. However, it is difficult to find natu- absorber with theoretical unity absorptivity realized through
rally existing materials with strong absorption coefficients that perfect impedance matching was demonstrated [13]. Progress
are also compatible with standard microfabrication techniques. has been made to extend the absorber design to terahertz
Thus, metamaterials are a promising approach to manipulate frequencies by using double metamaterial layers [14,
terahertz waves and to fill this terahertz gap [8, 9]. 15]. Although those metamaterial absorbers show decent
Sub-wavelength split ring resonators (SRRs) have been absorptivity at terahertz frequencies, they are basically single
extensively employed to exhibit a magnetic or electric band absorbers with high absorptivity at a specific frequency.
resonance response at terahertz frequencies [611]. Although Multi-band terahertz absorbers with two or more optimized
SRR structures are bianisotropic, it is possible to eliminate the absorption peaks have yet to be demonstrated, which could
magnetoelectric coupling by making symmetrical structures be important, for example, in the development of terahertz
such as electric-field-coupled (ELC) resonators with shared spectroscopic imagers/detectors [16, 17].
centre gap or shared centre bar. A pure electric resonance We experimentally demonstrate a dual band resonant
response was experimentally demonstrated at microwave metamaterial absorber with two distinct absorption peaks at
frequency with the EM wave propagating along the substrate 1.4 and 3.0 THz. We use an absorber design similar to [15].

0022-3727/10/225102+05$30.00 1 2010 IOP Publishing Ltd Printed in the UK & the USA
J. Phys. D: Appl. Phys. 43 (2010) 225102 H Tao et al

w
h1 g1

h2 g2
b 30 m
30m
a
(a) (b) (c)
Figure 1. Dual band terahertz metamaterial absorber consisting of a dual band ELC resonator and a metallic ground plane, separated by an
8 m thick dielectric layer. (a) Perspective view of the absorber. (b) Top view of the absorber. (c) Photograph of a portion of the fabricated
absorber. Corresponding dimensions are shown in table 1. (Colour online.)

The main difference is that we combine two single band across the entire frequency range. Thus, the absorptivity can
ELC resonators together to obtain the dual band resonance be calculated using A = 1 R, which makes optimizing the
responses, inspired by [18]. Remarkably, the two resonance absorptivity equivalent to minimizing the reflectivity. The
responses can be tuned and optimized independently at desired optimized parameters are those which yielded the lowest
frequencies with comparably high absorptivity as with single reflectivity at the design frequencies of 1.4 and 2.9 THz.
band metamaterial absorbers. This feature provides more As observed in [15], a metamaterial absorber based on a
flexibility in multi-band absorber designs and can be readily different kind of single ELC resonator, referred to as electric
extended to infrared and visible frequency ranges. SRR (e-SRR), also shows two absorption peaks at two distinct
As described in [14, 15], maximizing the absorption (A) frequencies. However, it is different from the dual band
is equivalent to minimizing both the transmission (T ) and the absorber due to the different origin of the absorption. The
reflectivity (R) simultaneously at the same frequency range. low frequency resonance is due to countercirculating currents
The near-unity resonant metamaterial absorber can be realized in the e-SRR, while the high frequency resonance derives from
by manipulating the effective and to get perfect impedance a dipolar response [19], analogous to what has previously
matching with free space (i.e. Z = Z0 , resulting in R = 0), been observed using frequency-selective surfaces (FSSs) at
with the loss dependent imaginary part of the refractive index microwave frequencies [20, 21]. In the dual band absorber,
(n2 ) as large as possible. both resonances come from circulating currents in the ELC
A dual band metamaterial absorber consists of two resonators, while the low frequency response is determined
metallic layers separated by a dielectric spacer. The top layer mainly by the upper resonator (S1) and the high frequency
consists of an array of dual band ELC resonators which is response is contributed mainly by the lower resonator (S2).
responsible for determining  (), while the bottom metallic This was verified by examining the surface current distribution
ground plane layer is added such that the incident magnetic on resonance, as shown in figures 2(c) and (d). The two
field drives circulating currents between the two layers, as resonance peaks are labelled as I (at 1.4 THz) and II (at
shown in figure 1. Two single band metamaterial absorbers 2.9 THz), respectively. To better understand the absorption
with only one single ELC resonator on the top layer are first of each resonance, an absorber based on e-SRR with centre
designed and optimized near 1.4 THz (S1) and 2.9 THz (S2), split gap (D1), similar to the design in [15], was designed and
and are then integrated into a single particle, as shown in optimized with similar absorption peaks as the dual band ELC
figure 2. Despite coupling between these two ELC resonators resonator absorber (D2) near 1.4 and 2.9 THz. In comparison
due to the shared bar (see D2), two distinct absorption peaks with the e-SRR absorber (D1), the dual band ELC absorber
are obtained by fine tuning of the overall geometry. (D2) has a similar low frequency response. However, it
The absorber structures were simulated and optimized has significantly higher and narrower resonance absorption
using commercialized full-wave EM simulation software CST response at the higher frequency.
Microwave Studio 2008. Unit cell boundary conditions An additional aspect to consider in the design of
with a tetrahedral mesh were used in the frequency solver, metamaterial absorbers is losses in the constituent materials
in which case the wave ports were automatically added in the making up the structure. As discussed in the introduction, one
direction of normal incidence to the substrate. The optimized of the design criteria is to obtain a large value of the imaginary
geometries are shown in table 1. The Au portions of the part of the effective refractive index. This necessitates having
absorbers were modelled as lossy gold with a conductivity some losses in the metal. Losses in the dielectric spacer are
= 4.09107 S cm1 , and the polyimide layer was modelled expected to contribute as well. For example, in the limit
using the experimentally determined value of  = 1 + i2 = of a perfect electric conductor and a lossless dielectric, the
2.88 + i0.09. The transmission amplitude S21 and reflection absorption in the composite in figure 1 is zero. However,
amplitude S11 were obtained and the absorption was calculated losses in gold are sufficient to yield a strong narrow band
using A = 1 R T = 1 S11 2
S21 2
, where S21 is zero resonance. The absorption as a function of frequency at various

2
J. Phys. D: Appl. Phys. 43 (2010) 225102 H Tao et al

(a) S1 S2
S2 E

Absorptivity
S1
I

(c)
(b) I II
E
Absorptivity

D2

k
g h II
D1
D1
D2

Frequency (THz) (d)


Figure 2. (a) and (b) show calculated absorptivity of the absorbers composed of S1 (red long dash), S2 (blue short dash), D1 (purple dot
line) and D2 (black solid line). (c) and (d) show simulated surface current density for the two absorptivity peaks on resonance with the
electric field (E) perpendicular to the resonatorsgap. (Colour online.)

Table 1. Dimensions of terahertz metamaterial absorbers (all units in m).


Sample a b w h1 h2 g1 g2 t h g k
S1 33.3 23.3 2 20.7 2 8
S2 33.3 23.3 2 8.7 2 8
D1 42.5 32.5 2 8 25 2 9
D2 33.3 23.3 2 18 7 2 2 8

Note: a, lattice period; b, outer dimension; w, line width; h1, height of S1; h2,
height of S2; g1, gap distance of S1; g2, gap distance of S2; t, thickness of the
polyimide spacer; h, height of D1; g, gap distance of D1; k, length of the gap
of D1.

values of the dielectric loss tangent tan() are calculated for the The dual band ELC absorber (D2) shows similar
metamaterial absorber designs D1 and D2, as shown in figure 3. absorption responses with various dielectric loss values at
The results in the figure start from a lossless dielectric both resonant frequencies as the e-SRR absorber (D1) does
(tan() = 0, black curve) and gradually increased tan() to 0.2 at low frequency. In the case of tan() = 0, the peak
(while keeping the value of the Au conductivity constant). The absorption is 0.86 at 1.4 THz and 0.84 at 2.9 THz, respectively,
e-SRR absorber (D1) shows different absorption responses at which are nearly 15% smaller than the calculation value in
two resonant frequencies with increasing tan() due to different figure 2(b). The absorption can be increased by increasing
resonant origins mentioned above. The peak absorption is 0.94 the dielectric losses, and it drops back after a certain value,
at 1.4 THz with a lossless dielectric, which is smaller than the which is 0.04 in this case. These results suggest that
calculated value in figure 2(b). This suggests losses in the optimization of tan() of the dielectric spacer can maximize
dielectric contribute to increasing the absorption. However, the metamaterial absorption. Further, it appears the losses
a point of diminishing returns is reached for larger values in polyimide (tan() = 0.031) should contribute 0.15 to
of tan() in that the absorption decreases and the resonance the absorption of our dual band metamaterial absorber as is
broadens. For the higher frequency resonance, the absorption evident by comparing the black curves in figures 2(b) and
keeps increasing with larger dielectric losses, which conforms 3(b). Besides optimization tan() of the dielectric spacer to
to those FSSs reported previously [22]. maximize the absorption, we can also optimize the absorber

3
J. Phys. D: Appl. Phys. 43 (2010) 225102 H Tao et al

(PI-5878G, HD MicroSystems) was spin-coated on the


(a) ground plane to form the 8 m thick polyimide spacer. Then
E the ELC resonator arrays were patterned with a conventional
lithography technology on the polyimide spacer. The lift
Absorptivity

off process was accomplished by e-beam evaporating another


D1 50 nm thick Au/Ti film, followed by rinsing in acetone for
several minutes. It is worth mentioning that the whole
fabrication process could be easily repeated at other substrates
including soft substrates such as polyimide to make it a
mechanically flexible dual band metamaterial absorber for
non-planar applications.
A Fourier transform infrared (FTIR) spectrometer was
0.00 used to experimentally verify the behaviour of the absorbers
(b) 0.04 by measuring the reflection response over the frequency range
0.08 of 13.4 THz with a resolution of 15 GHz. A liquid helium
0.12
cooled bolometer detector and a 6 m mylar beam splitter were
Absorptivity

0.20
used to optimize the FTIR performance over the frequencies
E measured. The absorber samples were diced into 1 cm 1 cm
squares and mounted with the electric field perpendicular to
the ELC resonator gaps. The samples were mounted on
D2
a commercially purchased reflection unit and the minimum
achievable incident angle for reflection measurements in
our current setup is constrained to 30 off-normal due to
the experimental limitations [23]. The measurements were
Frequency (THz) performed with an electric field perpendicular to the ELC
Figure 3. Calculated absorptivity as a function of frequency for resonator gap to excite the electric resonance. The absorption
various values of the dielectric loss tangent used in (a) single e-SRR spectrum was easily obtained from the reflection results.
metamaterial absorber D1 and (b) dual band ELC metamaterial The experimental results for all four absorbers are
absorber D2. The electric field (E) is aligned perpendicular to the
displayed in figure 4. For the single ELC resonator absorbers,
resonatorsgap. The curves are labelled with the value of tan() used
in the simulation. (Colour online.) S1 shows an absorptivity of 0.74 at 1.46 THz and S2 shows
an absorptivity of 0.93 at 2.99 THz, which is in reasonable
Table 2. Calculated absorptivity peaks of dual band metamaterial agreement with the simulation though the absorption peaks
absorber as a function of the dielectric loss tangent value and the are lower than expected partly due to fabrication imperfections.
spacer thickness.
For dual band resonator absorbers, D1 shows an absorptivity
Dielectric tan() t A1 (%) A2 (%) B1 (%) B2 (%) of 0.79 at 1.43 THz and another absorption peak of 0.86 at
1 0.00 5.5 85.81 83.97 99.97 99.75 2.95 THz; D2 shows two strong resonance absorption peaks of
2 0.04 8 99.96 99.81 99.96 99.81 0.85 at 1.41 THz and 0.94 at 3.02 THz. There is a noticeable
3 0.08 10 95.34 97.96 99.86 99.93 frequency shift (0.1 THz) at the high resonant frequency
4 0.12 12 87.25 92.85 99.64 99.64 between experimental and simulation results in D2, which
5 0.20 16 72.55 82.98 98.70 98.01
is mainly due to the inaccuracy of the fabricated resonator
Note: tan(), loss tangent of the dielectric spacer; t, modified gap distance. The off-resonance absorptivity (0.3) is quite
thickness of the dielectric spacer in m; A1, absorptivity peak large in disagreement with the simulations (0.1), which may
value at low frequency with 8 m thick dielectric spacer; A2, result partly from the scattering of radiation due to fabrication
absorptivity peak value at high frequency with 8 m thick
dielectric spacer; B1, absorptivity peak value at low frequency imperfections. Although the absorption peaks are lower than
with modified dielectric spacer thickness; B2, absorptivity peak the simulated values, it is clear that the absorber consisting
value at high frequency with modified dielectric spacer of dual band ELC resonators (D2) shows higher absorption
thickness. and better spectral resolution than the single e-SRRs (D1),
and therefore should be a better candidate to be included as
geometry for various dielectric spacers with different losses. an active absorbing element in spectrally selective terahertz
By simply tuning the thickness of the dielectric spacer without detectors.
having to modify the dual band ELC resonators geometry, In summary, a dual band terahertz metamaterial absorber
the absorption peaks can be pulled back to near unity at both consisting of two single ELC resonators combined together and
resonant frequencies, as shown in table 2. a metallic ground plane, separated by a dielectric spacer, has
The above-mentioned absorber structures were fabricated been demonstrated. Two distinct resonant absorption peaks at
on silicon substrates with the parameters shown in table 1. A 1.4 and 3.0 THz were experimentally observed, and the two
50 nm thick Au/Cr film was first e-beam evaporated on a 2 absorption peaks can be individually tuned by optimizing the
inch silicon wafer to form the ground plane. Liquid polyimide corresponding single ELC resonators geometries.

4
J. Phys. D: Appl. Phys. 43 (2010) 225102 H Tao et al

(a)

Absorptivity
S1

S1
S2 S2 (c)

(b)

D1 In
Absorptivity

Sample
Out
D1
D2 D2 (d)

Frequency (THz)

Figure 4. (a) and (b) Experimental absorptivity as a function of frequency. S1 (red long dash), S2 (blue short dash), D1 (purple dot line)
and D2 (black solid line). (Insets: photographs of portions of as-fabricated absorbers.) (c) Photo of the reflection unit used in the
measurement. (d) Schematic of the reflection measurement setup. (Colour online.)

Acknowledgments [9] Chen H T, OHara J F, Azad A K, Taylor A J, Averitt R D,


Shrekenhamer D and Padilla W J 2008 Nature Photon.
This project has been supported in part by the DOD/Army 2 295
[10] Padilla W J, Aronsson M T, Highstrete C, Lee M, Taylor A J
Research Laboratory under contract no W911NF-06-2-0040, and Averitt R D 2007 Phys. Rev. B 75 041102(R)
NSF under contract no ECCS 0802036, AFOSR under [11] Bingham C M, Tao H, Liu X, Averitt R D, Zhang X and
contract no FA9550-09-1-0708, and DARPA under contract Padilla W J 2008 Opt. Express 16 18565
no HR0011-08-1-0044. The authors would also like to thank [12] Schurig D, Mock J J and Smith D R 2006 Appl. Phys. Lett.
the Photonics Centre at Boston University for all the technical 88 041109
[13] Landy N I, Sajuyigbe S, Mock J J, Smith D R and Padilla W J
support throughout the course of this research. 2008 Phys. Rev. Lett. 100 207402
[14] Tao H, Landy N I, Zhang X, Averitt R D and Padilla W J 2008
Note added in proof. During the course of this work we were Opt. Express 16 7181
made aware of a paper with similar results [24]. [15] Tao H, Bingham C M, Strikwerda A C, Pilon D,
Shrekenhamer D, Landy N I, Fan K, Zhang X, Padilla W J
and Averitt R D 2008 Phys. Rev. B 78 241103(R)
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