Vol. 24, No.

20 | 3 Oct 2016 | OPTICS EXPRESS 22461

1 μJ, sub-300 fs pulse generation from a

compact thulium-doped chirped pulse
amplifier seeded by Raman shifted erbium-
doped fiber laser
FANGZHOU TAN, HONGXING SHI, RUOYU SUN, PENG WANG, AND PU
WANG*
Institute of Laser Engineering, Beijing University of Technology, Beijing Engineering Research Center
of Laser Applied Technology, Beijing 100124, China
*
wangpuemail@bjut.edu.cn

Abstract: We present a compact thulium-doped chirped pulse amplifier producing 241 fs

pulses with 1 μJ energy. The system is seeded with the Raman shifted soliton generated by
the combination of an erbium-doped femtosecond laser and a nonlinear fiber. The Tm-doped
large mode area fiber yields output power of 71 W, corresponding to pulse energy of 2.04 μJ,
with a slope efficiency of 52.2%. The amplified pulses have been compressed to a duration
time of 241 fs, using a folded Treacy grating setup. The pulse energy is measured to be 1.02
μJ, corresponding to a peak power of ~3 MW. To the best of our knowledge, this is the
highest average power and pulse energy generated from an all-fiber, Raman shifted soliton
seeded thulium-doped chirped pulse amplifier system.
© 2016 Optical Society of America
OCIS codes: (140.4050) Mode-locked lasers; (140.3510) Lasers, fiber; (140.3280) Laser amplifiers; (140.3538)
Lasers, pulsed; (320.5520) Pulse compression; (320.7090) Ultrafast lasers.

References and Links

1. C. W. Rudy, M. J. F. Digonnet, and R. L. Byer, “Advances in 2-μm Tm-doped mode-locked fiber lasers,” Opt.
Fiber Technol. 20(6), 642–649 (2014).
2. P. Kadwani, J. Chia, F. Altal, R. A. Sims, C. Willis, L. Shah, D. Killinger, and M. C. Richardson, “Atmospheric
absorption spectroscopy using Tm: fiber sources around two microns,” Proc. SPIE 7924, 79240L (2011).
3. K. D. Polder and S. Bruce, “Treatment of melasma using a novel 1,927-nm fractional thulium fiber laser: a pilot
study,” Dermatol. Surg. 38(2), 199–206 (2012).
4. I. Mingareev, F. Weirauch, A. Olowinsky, L. Shah, P. Kadwani, and M. Richardson, “Welding of polymers
using a 2 μm thulium fiber laser,” Opt. Laser Technol. 44(7), 2095–2099 (2012).
5. F. Adler and S. A. Diddams, “High-power, hybrid Er:fiber/Tm:fiber frequency comb source in the 2 μm
wavelength region,” Opt. Lett. 37(9), 1400–1402 (2012).
6. C. W. Rudy, A. Marandi, K. L. Vodopyanov, and R. L. Byer, “Octave-spanning supercontinuum generation in
in situ tapered As2S3 fiber pumped by a thulium-doped fiber laser,” Opt. Lett. 38(15), 2865–2868 (2013).
7. K. Liu, J. Liu, H. Shi, F. Tan, and P. Wang, “High power mid-infrared supercontinuum generation in a single-
mode ZBLAN fiber with up to 21.8 W average output power,” Opt. Express 22(20), 24384–24391 (2014).
8. N. Leindecker, A. Marandi, R. L. Byer, K. L. Vodopyanov, J. Jiang, I. Hartl, M. Fermann, and P. G.
Schunemann, “Octave-spanning ultrafast OPO with 2.6-6.1 µm instantaneous bandwidth pumped by
femtosecond Tm-fiber laser,” Opt. Express 20(7), 7046–7053 (2012).
9. M. Gebhardt, C. Gaida, F. Stutzki, C. Jauregui, J. Limpert, and A. Tünnermann, “Sub-200 fs, nJ-level stretched-
pulse thulium-doped fiber oscillator at 23MHz repetition rate,” in Advanced Solid State Lasers, OSA Technical
Digest (online) (Optical Society of America, 2014), paper AM5A.43.
10. M. Gebhardt, C. Gaida, F. Stutzki, S. Hädrich, C. Jauregui, J. Limpert, and A. Tünnermann, “Impact of
atmospheric molecular absorption on the temporal and spatial evolution of ultra-short optical pulses,” Opt.
Express 23(11), 13776–13787 (2015).
11. R. Gumenyuk, I. Vartiainen, H. Tuovinen, and O. G. Okhotnikov, “Dissipative dispersion-managed soliton 2
μm thulium/holmium fiber laser,” Opt. Lett. 36(5), 609–611 (2011).
12. A. Wienke, F. Haxsen, D. Wandt, U. Morgner, J. Neumann, and D. Kracht, “Ultrafast, stretched-pulse thulium-
doped fiber laser with a fiber-based dispersion management,” Opt. Lett. 37(13), 2466–2468 (2012).
13. F. Haxsen, D. Wandt, U. Morgner, J. Neumann, and D. Kracht, “Monotonically chirped pulse evolution in an
ultrashort pulse thulium-doped fiber laser,” Opt. Lett. 37(6), 1014–1016 (2012).
14. J. P. Gordon, “Theory of the soliton self-frequency shift,” Opt. Lett. 11(10), 662–664 (1986).

#272983 http://dx.doi.org/10.1364/OE.24.022461
Journal © 2016 Received 3 Aug 2016; revised 12 Sep 2016; accepted 12 Sep 2016; published 19 Sep 2016
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22462

15. G. Imeshev and M. Fermann, “230-kW peak power femtosecond pulses from a high power tunable source based
on amplification in Tm-doped fiber,” Opt. Express 13(19), 7424–7431 (2005).
16. R. Herda and A. Zach, “All-fiber generation of few-cycle pulses at 1950 nm by triple-stage compression of a
Thulium-doped laser system,” in Proceedings of IEEE Conference on Photonics Conference (IEEE, 2013), pp.
621–622.
17. C. Gaida, M. Gebhardt, F. Stutzki, C. Jauregui, J. Limpert, and A. Tünnermann, “Thulium-doped fiber chirped-
pulse amplification system with 2 GW of peak power,” Opt. Lett. 41(17), 4130–4133 (2016).
18. F. Tauser, F. Adler, and A. Leitenstorfer, “Widely tunable sub-30-fs pulses from a compact erbium-doped fiber
source,” Opt. Lett. 29(5), 516–518 (2004).
19. A. Sell, G. Krauss, R. Scheu, R. Huber, and A. Leitenstorfer, “8-fs pulses from a compact Er:fiber system:
quantitative modeling and experimental implementation,” Opt. Express 17(2), 1070–1077 (2009).
20. S. Kumkar, G. Krauss, M. Wunram, D. Fehrenbacher, U. Demirbas, D. Brida, and A. Leitenstorfer,
“Femtosecond coherent seeding of a broadband Tm:fiber amplifier by an Er:fiber system,” Opt. Lett. 37(4),
554–556 (2012).
21. D. Brida, G. Krauss, A. Sell, and A. Leitenstorfer, “Ultrabroadband Er:fiber lasers,” Laser Photonics Rev. 8(3),
409–428 (2014).
22. R. A. Sims, P. Kadwani, A. S. Shah, M. Richardson, and M. Richardson, “1 μJ, sub-500 fs chirped pulse
amplification in a Tm-doped fiber system,” Opt. Lett. 38(2), 121–123 (2013).
23. M. E. Fermann, V. I. Kruglov, B. C. Thomsen, J. M. Dudley, and J. D. Harvey, “Self-similar propagation and
amplification of parabolic pulses in optical fibers,” Phys. Rev. Lett. 84(26), 6010–6013 (2000).
24. Y. Kim, Y. J. Kim, S. Kim, and S. W. Kim, “Er-doped fiber comb with enhanced fceo S/N ratio using Tm:Ho-
doped fiber,” Opt. Express 17(21), 18606–18611 (2009).

1. Introduction
Pulsed 2 μm fiber laser sources have attracted intense interests in recent years [1] for its wide
applications in remote sensing [2], medicine [3], plastic engineering [4], mid-IR frequency
comb [5], nonlinear mid-IR supercontinuum generation [6,7], optical parametric generation
[8] and so on. To produce picosecond or femtosecond pulses at 2 μm wavelength regime,
mode-locking and nonlinear frequency conversion are two major approaches. Thulium fiber
based mode-locked oscillators are usually operating at the wavelengths below 2 μm, which
may be affected by water absorption around 1.9 μm [9,10]. Because the material dispersion
values of silica glass around 2 μm is positive and relatively high, to generate pulses with
pulse durations from picoseconds to hundreds of femtoseconds and repetition rates of MHz,
normally dispersion-managed mode-locked thulium-doped fiber lasers are employed [11–
13]. Using erbium-doped femtosecond fiber lasers to generate Raman shifted solitons have
been proved to be a powerful and effective way to obtain ultrafast pulses at 2 μm regime, in
comparison with the alternative 2 μm mode-locked oscillators. This is because the well-
developed 1.5 μm fiber-based components are mature, stable and costless. The center
wavelength of the generated Raman solitons beyond 1.5μm can be shifted by controlling the
pumping power level [5,14–16,18–21]. This can be achieved through either the soliton self-
frequency shift (SSFS) [14,15] or spectral broadening in highly nonlinear fibers [5,16,18–
21]. So far, the shortest pulse width of 27 fs has been achieved using this approach, with
three additional compression stages at 2 μm [16].
However, there are still some drawbacks for this kind of sources. For example, extra
noises can be introduced from the nonlinear frequency generation processes [5], and the
configuration of the laser source can be complex compared with thulium doped mode-
locking oscillators. Moreover, the Raman-shifted source usually delivers pulse energy of pJ-
to nJ-level, which is an obvious barrier to extend this sort of sources for some applications
requiring higher pulse energy.
For further power scaling, nonlinear amplification and chirped pulse amplification (CPA)
are the two common ways to generate 2 μm high-energy pulses with sub-ps pulse duration.
To date, the highest reported pulse energy is 31 nJ using the nonlinear amplification
approach, seeded by the Raman shifted soliton from an ultrafast erbium-doped fiber laser
[15]. In that work, the shifted Raman soliton pulses were positively pre-chirped by a segment
of normal dispersion fiber (NDF), before being amplified in a thulium-doped large mode area
(LMA) fiber. Pulses with a width of 108 fs were obtained during the nonlinear amplification
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22463

with center wavelength of 1980 nm. However, there is a trade-off between the fiber
nonlinearity and the dispersion during the nonlinear amplification. This limits the achievable
pulse energy since excessively high nonlinearity will cause pulse breakup.
On the other hand, pulse energy of 470 μJ with peak power up to 2 GW has been realized
in thulium-doped chirped pulse amplification system seeded by 2 μm thulium-doped fiber
oscillator. The generation of the pulses with such high energy is benefited from the usage of
a large-pitch thulium-doped fiber, as well as complex free-space stretchers and high
efficiency grating compressors [17].
Insteadly, R. A. Sims et al reported chirped pulse amplification seeded by Raman soliton
pulses from a 1.9 μm mode-locked thulium doped fiber laser [22]. The shifted Raman
solitons were positively stretched by a chirped Bragg grating (CBG). The pulse repetition
rate is then reduced down to 100 kHz by an electro-optic modulator. After the amplification
of a thulium-doped LMA fiber and the compression of grating pairs, pulses with energy of 1
μJ and pulse width below 500 fs were finally obtained. The CBG in the experiment was also
used as spectral filter to remove the unwanted spectral portion lying in the thulium gain
bandwidth. However, the system is not an all-fiber device, due to the insertion of the free-
space CBG stretcher. This makes the system complex and inconvenient.
In this work, we demonstrate a compact all-fiber thulium-doped chirped pulse
amplification system seeded by a Raman-shifted erbium-doped fiber laser. The average
output power of the amplified pulses was measured to be 71 W with a slope efficiency of
52.2%. The repetition rate has been measured to be 34.8 MHz. The pulses are then
compressed to a duration time of 241 fs with 35.4 W average output power corresponding to
a peak power of ~3 MW.
2. Experimental setup

Fig. 1. Experimental setup of thulium-doped CPA system. ISO: isolator; TDF: thulium-doped
fiber; LMA-TDF: large mode area thulium-doped fiber.

The schematic setup of Tm-doped fiber CPA system is shown in Fig. 1. It consists of an all
fiber Raman soliton generator, a fiber stretcher, two stages of fiber amplifiers and a free-
space grating compressor. The Raman soliton generator is based on an amplified mode-
locked erbium-doped fiber (EDF) laser and a short piece of highly nonlinear fiber (HNLF).
The mode-locked EDF laser consists of a wavelength division multiplexer (WDM), a 20%
output coupler, a fiber optical circulator coupled with a commercial available SESAM
(semiconductor saturable absorber mirror) mode locker and a piece of EDF with the
dispersion of −12 ps/nm/km at 1550 nm. The total cavity length is about 5.75 m, which
corresponds to 34.8 MHz fundamental repetition rate. A fiber polarization controller (PC) is
placed before the amplification stage to optimize the compression pulse quality. The
amplifier consists of ~4 m EDF with the same parameters as the oscillator gain fiber. After
amplification, the pulses are compressed with 110 cm single mode fiber (SMF-28). A short
segment of HNLF was spliced directly to the SMF-28 fiber to generate the supercontinuum.
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22464

The HNLF has a mode field diameter of 2.23 μm, a dispersion of 2.187 ps/nm/km at 1550
nm, and a nonlinearity γ of ~9 W−1km−1 respectively. An additional 16 cm-long Tm:Ho-
doped fiber (TH512, Coractive Inc.) is used to further enhance the signal intensity at 2010
nm. Then the enhanced Raman soliton pulses are temporally stretched using ~110 m
ultrahigh numerical aperture fiber (UHNA-4, Nufern Inc.) with a dispersion of ~-48.5
ps/nm/km at 1.9 μm and amplified in two-stage thulium-doped fiber amplifier. The pre-
amplifier consists of a 3.5 m-long double clad single mode thulium-doped fiber (TDF). The
TDF is with a core diameter of 10 μm, an outer diameter of 130 μm (Nufern Inc.), and an NA
of 0.46 for the second cladding with cladding absorption of ~3 dB/m at 793 nm. A
commercial pump combiner is used to deliver pump light to the gain fiber from the
multimode pump diode, which has a center wavelength of 793 nm and output power of 12 W
with 0.22 NA, 105/125 μm fiber pigtail. In the main amplifier stage, 1.9 m LMA thulium
doped fiber (Nufern Inc.) is used to boost the signal power to tens of watts. The active fiber
has a core diameter of 25 μm, an NA of 0.09, an inner cladding diameter of 250 μm and a
cladding NA of 0.46 with cladding absorption of ~9.5 dB/ m at 793 nm. The active fiber is
water-cooled down to 12 °C to dissipate the heat accumulation as well as promoting efficient
two-for-one cross-relaxation during high power operation. The pump source consists of 5
diodes operating at 793 nm with 105 μm (NA = 0.22) pigtail fibers. The total output power of
these pump diodes is ~148 W. A (6 + 1) × 1 high power pump combiner (ITF Technologies
Inc.) is used to deliver pump light to the gain fiber with a coupling efficiency of ~95%. The
output end of the LMA thulium-doped fiber was angle cleaved to frustrate parasitic lasing.
After amplification a dichroic mirror (DM) is used to filter the unabsorbed pump light and
the pulses are compressed with a folded Treacy grating compressor consisting of two 560
grooves per mm, fused silica transmission gratings. A fused silica wedge is placed after the
compression output to measure the optical and radio-frequency (RF) spectra as well as pulse
characteristics.
3. Experimental results
The oscillator is a passively SESAM mode-locked erbium-doped fiber laser operating at
stretched pulse mode-locking regime. The net dispersion of the cavity is estimated to be
−0.048 ps2. The oscillator delivers an average output power of 1.5 mW with a pulse width of
1.1 ps and a repetition rate of 34.8 MHz. The output spectrum is shown in Fig. 2 (as the black
line) with a center wavelength of 1559 nm and a spectrum bandwidth of 12 nm, indicating
that the pulses are negatively chirped. The output pulses are amplified to about 68 mW by the
erbium-doped fiber amplifier (EDFA). The combination of the distributed gain, the normal
dispersion of the EDFA as well as self-phase modulation (SPM) effect leads to self-similar
amplification with appropriate input pulse energy, in which the pulses have been evolved to
parabolic shape with linear chirp [23]. After amplification, the width of the spectrum expands
to over 80 nm with nearly parabolic shape (see the red line in Fig. 2) and the amplified pulse
width is measured to be 1.15 ps. In the experiment, the SMF-28 with anomalous dispersions
is used to compress the chirped pulses. By carefully tailoring the SMF-28 fiber length with
cutback method, the pulse compression is maximized when the SMF-28 length is 110 cm.
The pulse duration after the compression fiber is measured to be ~70 fs and the bandwidth of
the compressed pulse spectrum (as the blue line shown in Fig. 2) is ~84 nm.
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22465

Fig. 2. Spectral traces of the erbium-doped fiber oscillator, amplifier and compressor.

An optimized short (13 cm) segment of HNLF is spliced with the SMF-28 to generate
Raman shifted solitons through nonlinear spectral broadening process. The generated
supercontinuum is recorded by an optical spectral analyzer (YOKOGAWA AQ6375). A
broad and smooth supercontinuum spectrum ranging from 1.2 to 2.1 μm is generated after the
HNLF under suitable pump power, (see the pink line in Fig. 3). The spectral broadening is
dominated by soliton fission and soliton self-frequency shifting, as we can see the separated
solitons at longer wavelength. The spectrum peak near 1950 nm is caused by the unabsorbed
976 nm pump signal. The supercontinuum can be further extended to beyond 2.3 μm with the
highest pump power in the experiment (see the orange line in Fig. 3). The pump power has
been optimized to generate Raman shifted soliton at the center wavelength of 2 μm, which is
away from the water vapor absorption in the air near the 1.9 μm regime. This is important
because the final stage of pulse compression is in the free space. The generated Raman
soliton is centered at ~2010 nm with a full width half maximum (FWHM) bandwidth of ~93
nm. As we can see from the output spectrum, most of the spectral power remains near the
wavelength between 1.5 and 1.7 μm. In order to fully utilize such residual spectral power and
enhance the signal intensity at 2010 nm, the supercontinuum output is then coupled into a 16
cm Tm:Ho-doped fiber (TH512, Coractive Inc.) to achieve self-amplification process [24].
The enhanced Raman soliton supercontinuum is shown in Fig. 3 (see the blue line).

Fig. 3. Spectra of the generated supercontinuum before (pink line) and after (blue line)
Tm:Ho-doped fiber, the generated supercontinuum at highest pump power (orange line) and
the amplified Raman pulses after LMA Tm-doped fiber (olive line).

Before the supercontinuum entered in the thulium doped fiber pre-amplifier, the Raman
shifted pulses are temporally stretched to ~320 ps to avoid the nonlinearities in the amplifier
introduced by high peak intensities inside the gain fiber. The output spectral power from
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22466

1900 nm to 2100 nm is estimated to be ~5 mW after the fiber stretcher. The stretched pulses
are amplified in the first stage thulium-doped fiber amplifier. An output power of ~850 mW
has been achieved after the isolator, with a pump power of ~7.6 W corresponding to a gain of
22 dB. Compared with the Raman soliton seed source, the spectrum bandwidth of the
amplified pulses was decreased to 42 nm due to the gain narrowing after the amplification
process. The center wavelength of the amplified pulses shows blue-shifted to 1984 nm
because of the thulium gain location. The pulse width of the amplified Raman solitons
decreases to ~180 ps with the narrowing of the amplified spectrum width. Due to the long
pulse duration in the gain fiber, no significant spectral distortion was observed at this stage.

Fig. 4. Output power (black square point) and output power after compression (red circle dot)
as a function of pump power in the final power amplifier.

The pre-amplified pulse train is further injected into the second amplifier for power
scaling. Spectral modulation has been observed after the pre-amplified pulses passing
through the LMA Tm-doped fiber, which is shown in Fig. 3 (see the olive line). This is
probably due to the multimode interference (MMI) in the LMA gain fiber [22]. Benefiting
from the high absorption of the gain fiber, short fiber length can be expected to obtain high
optical-to-optical power conversion efficiency and minimize nonlinear effects such as
stimulated Brillouin scattering and stimulated Raman scattering. Figure 4 shows the average
output power of the thulium-doped fiber power amplifier versus incident pump power. The
maximum average power and the corresponding pulse energy of the output are measured to
be 71 W (i.e., a gain of 18.9 dB) and 2.04 μJ respectively, when the incident pump power is
141 W. The average power increases linearly with the incident pump power with a slope
efficiency of ~52.2%. No amplified spontaneous emission has been observed during the
power amplification.
At the final stage, the amplified pulses are compressed by a folded Treacy compressor.
The compressor has a slope efficiency of 49.8% (see Fig. 4), which is mainly limited by the
diffraction efficiency of the gratings. The output power of the compressed pulses is measured
to be 35.4 W, corresponding to pulse energy of 1.02 μJ, at the maximum pump power of 141
W. The optical spectrum of compressed pulses is shown in Fig. 5(a), with a FWHM of 28.4
nm at the center wavelength of 1970 nm. The output spectrum is not smooth with some
modulation, we attribute this to the MMI in the LMA Tm-doped fiber and nonlinearities
generated at high pulse energies.
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22467

Fig. 5. (a) Output optical spectrum of the compressed pulses measured at highest pulse
energy. Inset: the output spectrum with logarithmic scale; (b) Autocorrelation trace of the
compressed pulse with 1.02 μJ output pulse energy.

Figure 5(b) illustrates the autocorrelation trace of the compressed pulses measured by a
commercial second harmonic generation (SHG) autocorrelator (Femtochrome, FR-103XL) at
the highest output power. The pulse duration after compression is 241 fs given a sech2 pulse
intensity profile. The time bandwidth product (TBP) is calculated to be 0.53. The pedestal is
seen in the autocorrelation trace. The formation of the pedestal can be attributed to the
nonlinear phase shifts generated in the Raman shift processing, the uncompensated high-
ordered dispersion of the stretcher fiber and the nonlinearities accumulated in the LMA fiber
amplifier under high power operation. According to the area integral in Fig. 5(b), the pulse
contains ~70% of the energy and the peak power is calculated to be ~3 MW. The average
output power has been continuously measured for 5 minutes and the variation is less than
1%, indicating excellent power stability of the compressed pulses.

Fig. 6. M2 measurement performed using a scanning slit beam profilers system. Inset, near-
field beam intensity profile at average output power of 70 W.

The output beam quality was measured using a scanning slit beam profilers system
(BeamScope-P8). A near-field intensity profile of the laser beam is shown in Fig. 6. The
beam quality factor M2 was measured to be 1.214 at average output power of 70 W.
 Vol. 24, No. 20 | 3 Oct 2016 | OPTICS EXPRESS 22468

Fig. 7. Measured RF spectra of the compressed pulsewith 1 MHz span and resolution of 300
Hz.

Figure 7 shows the RF spectrum (after compression) measured by a spectrum analyzer

(Agilent N9030A) and a 12.5 GHz InGaAs photodetector (Newport Inc.) at a span range of 1
MHz with the resolution bandwidth of 300 Hz. High signal-to-noise ratio of ~67 dB is
observed without visible sidebands, indicating low amplitude fluctuations between pulses.
4. Conclusions
In conclusion, we have reported a compact thulium-doped chirped pulse fiber amplifier
system, seeded by Raman shifted erbium-doped fiber laser. Output power of 71 W has been
achieved from the LMA fiber amplifier with a slope efficiency of 52.2%. The chirped pulses
are finally compressed to the duration time of 241 fs with the average power of 35.4 W,
corresponding to ~3 MW peak power. The generated smooth and ultra-broad band spectrum
of Raman shifted solitons indicates that it is a suitable seed source for multi-stage amplifiers.
Funding Information
National Natural Science Foundation of China (NSFC) (61527822, 61235010).
Acknowledgments
The authors acknowledge funding support from the Natural National Science Foundation of
China.