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International Wood Products Journal

ISSN: 2042-6445 (Print) 2042-6453 (Online) Journal homepage: https://www.tandfonline.com/loi/ywpj20

Binderless boards made of milled coconut husk:


an analysis of the technical feasibility and process
restraints

Thomas Böger, Sauro Bianchi, Corinna Salzer & Frédéric Pichelin

To cite this article: Thomas Böger, Sauro Bianchi, Corinna Salzer & Frédéric Pichelin (2018)
Binderless boards made of milled coconut husk: an analysis of the technical feasibility and process
restraints, International Wood Products Journal, 9:1, 3-8, DOI: 10.1080/20426445.2017.1400756

To link to this article: https://doi.org/10.1080/20426445.2017.1400756

Published online: 22 Nov 2017.

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INTERNATIONAL WOOD PRODUCTS JOURNAL, 2018
VOL. 9, NO. 1, 3–8
https://doi.org/10.1080/20426445.2017.1400756

Binderless boards made of milled coconut husk: an analysis of the technical


feasibility and process restraints
Thomas Bögera, Sauro Bianchia, Corinna Salzerb,c and Frédéric Pichelina
a
Institute for Materials and Wood Technology, Bern University of Applied Science, Biel/Bienne, Switzerland; bChalmers University of
Technology, Gothenburg, Sweden; cBase Builds, Singapore

ABSTRACT ARTICLE HISTORY


The possibility of producing binderless panels made of milled coconut husk, a largely available Received 19 June 2017
by-product of the coconut oil industry, has been shown in previous researches. Long pressing Revised 20 October 2017
times and a high risk of blisters have however hindered the industrial implementation of the Accepted 31 October 2017
process. In this study, a more energy-efficient manufacturing process, involving a tailored
KEYWORDS
degassing step, was developed on a laboratory scale and then validated at an industrial size Coconut husk; binderless
(2 × 1 m2). To achieve mechanical properties close to the European and Japanese standards board; hot pressing;
for fibreboards and to avoid the delamination of the boards, final densities between 900 and fibreboard
1000 kg m−3 had to be targeted. Similarly, a successful board production was only possible if
the moisture content of the husk was between 10 and 25%. The need for a suitable mat-
forming technology to avoid the risk of warping of the panel was highlighted.

Introduction
boards made of coconut husk without any adhesives
The coconut palm (Cocos nucifera [L.]) is a tree species was first reported by Hadinoto (1957). Since then,
which grows in Asia, Africa, Latin America, the Carib- manufacturing processes and properties of binderless
bean and the Pacific region. In 2013, the production of panels based on different raw materials have been
coconut fruits was estimated to be 62.5 million tonnes described in a large number of papers: e.g. bagasse
worldwide of which almost 15.5 million is from the pith (Mobarak et al. 1982; Nonaka et al. 2013), oil
Philippines (FAOSTAT 2015). The thick mesocarp of palm trunk (Hashim et al. 2010), kenaf core (Okuda
the fruit (Figure 1(a)), commonly known as husk, rep- and Sato 2004). The self-cohesion process has been
resents approximately 35% by weight of the fruit, and related to different and interdependent mechanisms,
represents a by-product of the coconut oil industry such as the softening and flowing of cell-wall polymers
that has limited exploitation. It contains approximately like lignin as they go beyond the glass transition temp-
30% of coconut fibres, called coir, and 70% of a spongy erature, and the thermal degradation of wood constitu-
and brittle matrix called pith, predominantly rep- ents to reactive volatiles (e.g. aldehydes) which are able
resented by parenchyma cells (van Dam, van den to cross-link lignin and other phenolics extractives
Oever, Teunissen, et al. 2004 – Figure 1(b)). While (Pintiaux et al. 2015). In the case of coconut husk,
the coir is seldom used for the manufacturing of bed- which is very rich in syringyl lignin, it was shown
ding, mats, yarn, ropes and riverbank stabilisation that upon heating, the material showed a typical exo-
(Ganchero and Manapol 2007; Ramadhas et al. therm around 140°C which disappears in a second
2008), the pith remains a low-value leftover. heating cycle (van Dam, van den Oever, Teunissen,
Wood-based panels in the Philippines are today et al. 2004). This irreversible change was related to a
mainly imported due to the lack of a domestic pro- thermosetting reaction of the lignin, which under con-
duction. Such imported materials, mostly plywood, trolled thermal conditions (e.g. above 140°C) might
are not affordable to the low-income population. then work as a natural binder. Binderless board pro-
Exploitation of the coconut husk as a raw material duction has in fact been generally performed at temp-
for the manufacturing of low-priced domestic fibre- eratures between 180 and 260°C (Pintiaux et al. 2015)
board might therefore represents a concrete opportu- often in combination with relatively long pressing fac-
nity for the Philippines. tors (60–300 s mm−1) and high pressures (5–12 MPa).
First reports on panels made of coconut husk and The most extensive attempts in the manufacturing
bound with adhesive were found in 1944 (Anonymous of binderless coconut husk boards were described by
1944). Several following attempts were reported in van Dam, van den Oever, and Keijsers (2004) and Snij-
Youngquist et al. (1994). The possibility of producing der et al. (2005). In these studies, boards with densities

CONTACT Sauro Bianchi sauro.bianchi@bfh.ch


© 2017 IWSc, The Wood Technology Society of the Institute of Materials, Minerals and Mining
4 T. BÖGER ET AL.

methyl bromide for 24 h, and delivered by airfreight


to Switzerland. The husk was then kiln-dried at 60°C
for 48 h until 15% in moisture content (MC). This
moisture content corresponded approximately to the
equilibrium MC of coconut husk in the mean climate
conditions in the Philippines (30°C – 80% relative
humidity). The husk was thereafter hammer milled
with a 5 mm screen. During hammer milling the pith
Figure 1. Coconut fruit morphology: (a) coconut nut sur-
was powdered to very fine particles and partially lost
rounded by its mesocarp (husk); (b) SEM picture of a coconut
husk fibre embedded in parenchyma cells (pith). in the dust extraction system. Sieving analysis of the
milled husk showed that approximately 65% w/w of
the particles was below 0.310 mm, and nearly 50% w/w
between 1200 and 1300 kg m−3 were produced with a between 0.125 and 0.310 mm. The length of the milled
batch operating hot press. The high density of the fibres was approximately between 5 and 20 mm.
boards hindered the release of the steam pressure
developed during the pressing: delamination cracks
and blisters were consequently frequently observed. Mat forming
To solve this issue, the boards were cooled under The milled coconut husk was fluffed in a drum blender
pressure inside the press. A continuous cooling and to ensure a homogeneous distribution of fibres and
reheating of a batch press is obviously not energy-effi- pith. A mat was then formed by hand inside a wooden
cient at an industrial scale, and similar production con- frame, taking care to avoid an uneven distribution of
ditions are unrealistic to be performed on a continuous the husk throughout the mat and the separation of
press. Furthermore, the required pressing load the pith from the fibres. The density of the mat before
(>10 MPa) needed special equipment to be safely pressing was between 90 and 100 kg m−3. A K-type
applied at the industrial scale. As a consequence, the thermocouple was placed in the centre of the mat to
developed process did not succeed to be turned into record the middle-layer temperature during the hot
an actual industrial production. pressing.
In this study, an alternative hot pressing process for
producing binderless boards made of coconut husk
without the need of the final cooling was developed. Hot pressing
A controlled degassing phase was introduced during
A hot pressing cycle for the manufacturing of coconut
the pressing, inspired by similar solutions applied in
husk panels of 5 and 12 mm in thickness was prelimi-
the production of wood-based hardboards (Dunky
nary developed using a laboratory scale hot press
and Niemz 2002). The developed pressing cycle was
(HLOP210 Höfer Presstechnik GmbH – Austria).
applied and optimised on a pilot industrial-scale
The most suitable hot plate temperature range for the
plant (2 × 1 m2). Possibilities and limitations of the
production of the binderless panels was identified to
developed process were discussed.
be between 170 and 190°C.
Higher temperatures increased the risk of delamina-
Materials and methods tion, while lower temperatures were not enough for
reaching a sufficient mechanical binding between
Coconut husk
husk particles. The need for a degassing phase during
Coconut husks from the variety Laguna Tall were har- the hot pressing, to partially release the developed
vested in the Luzon region, sun dried, fumigated with steam pressure inside the boards, was evidenced.

Figure 2. Thickness cross section of a 12 mm thick binderless panel made of milled coconut husk.
INTERNATIONAL WOOD PRODUCTS JOURNAL 5

on both sides. The mechanical and physical properties


of the panels were measured and evaluated according
the following guidelines:

. EN 310:1993 = flexural modulus (modulus of elas-


ticity – MOE) and flexural strength (modulus of
rupture – MOR)
. EN 319:1993 = tensile strength perpendicular to the
plane of the board (internal bond – IB)
. EN 317:1993 = thickness swelling (TS)

The mean density of each specimen was first


measured according to the guideline EN 323:1993.
Density profiles along the thickness were measured
by X-ray absorption using a DAX 5000 (Grecon) device
with internal calibration.
Figure 3. Pressure, middle-layer temperature and press plate
distance used in the industrial production for a 5 mm panel
(2 × 1 m2) with a target density of 1000 kg m−3. Results and discussion

The developed pressing cycle was then applied and Panel production
optimised on an industrial size (1 × 2 m2) hot pressing The developed pressing cycle permitted the production
plant at Dieffenbacher GmbH (Eppinger, Germany) of 5 mm thick coconut husk panels in about 6.5 min at
heated to 170°C. Three industrial-scale coconut husk the industrial scale. No cooling step was needed at the
panels of 5 mm in thickness and 1000 kg m−3 density end of the process, substantially reducing therefore
were produced according to the pressing cycle dis- both the production time (30 min) and the energy con-
played in Figure 3. Trials using different press con- sumption in comparison to previous works (Snijder
ditions and/or other target densities were also made. et al. 2005). Similar pressing cycles including initial
A total of 10 panels were produced. The developed degassing were used successfully in the production
press cycle consisted of a quick initial closing to of kenaf core binderless boards (Okuda and Sato
9 mm, followed by a slower movement to a thickness 2004), but with a significantly longer pressing time
10% higher than the target value (5.5 mm) and holding (11 min). 12 mm thick panels were also produced
of this position for 150 s. These steps permitted the showing a compact thickness cross section (Figure 2).
necessary temperature of 150°C to be quickly reached In this case the press cycle had to be prolonged to
in the middle layer of the panel as determined van 13 min, in order to permit the middle layer to reach
Dam, van den Oever, Teunissen, et al. (2004), to start 150°C, conditions that are needed for starting of the
the thermosetting curing of the husk lignin. Concur- thermosetting behaviour of the lignin.
rently, the steam developed inside the panel had the Furthermore, the maximum pressure reached
possibility to outflow easily through the panel before during the pressing of 1000 kg m−3 density panels
it reached the final high compactness. In the next was always lower than 4 N mm−2, much less than the
step the press was closed to the target thickness 9.5 N mm−2 reported by Snijder et al. (2005) even if
(5 mm) and held in this position for about 250 s. for significantly denser panels (1200 kg m−3). The
During the last 2 min of the cycle, the press was reduction of the maximum pressure in the manufactur-
switched from position to pressure steering and the ing process would then allow the use of the same press-
load released at a rate of 0.5 MPa min−1. ing equipment as for standard wood-based fibreboards,
Two 12 mm thick industrial-scale panels with a tar- without the need for customised presses.
get density of 1000 kg m−3 were also produced using an Some boundaries in the pressing conditions were
analogous press cycle. Three other panels with lower observed during the press cycle development. An
densities were also produced. To compensate for the increase in the moisture content (MC) of the milled
higher thickness of the panel the initial and second coconut husk over 25%, even though it permitted a
holding steps were increased to 400 and 300 s, slightly faster heating of the middle layer (because of
respectively. the boosted heat convection (Deppe and Niemz
1996), brought the risk of blister and delamination to
unacceptable levels.
Mechanical and physical properties
The reduction of the husk MC to 6% also resulted in
After production and air cooling at room temperature, panels with a lack of compactness and poor binding
all the manufactured panels were sanded about 0.2 mm between particles. This result is in agreement with
6 T. BÖGER ET AL.

Figure 4. Warped and delaminated coconut husk binderless panel.

previous studies that evidenced the need for a mini- towards the lower surface during the mat forming,
mum level of MC in binderless processes (Nadhari leaving a fibre-richer layer at the upper surface. The
et al. 2013) and identified an optimum working win- need for a customised mat-forming system for the
dow in the MC range between 10 and 30% (Okuda milled coconut husk was therefore highlighted in
and Sato 2004). view of an industrial implementation of the process.
Panels with a target density higher than
1000 kg m−3 could not be produced. In fact above
Mechanical properties
this density, delamination was frequently observed
(Figure 4), most likely due to the high compactness The MOR, MOE and IB of 5 mm thick coconut
of the material that did not permit a sufficient release husk boards were measured on 138 samples each
of the steam pressure. retrieved from boards of average densities between
During the panel production, warping of panels 734 and 1156 kg m−3. MOR ranged between 4.4
occasionally occurred. It is likely that an uneven and 37.4 N mm−2 and MOE between 467 and
material distribution as well as local variations of the 4762 N mm−2. Both factors showed a distinct linear
fibre/pith ratio in the cross section and in the plane correlation (R 2 = 0.827 and 0.844, respectively) with
of the panel caused internal stresses during the pro- the panel density in the range between 700 and
duction. Density profile measurements on samples col- 1200 kg m−3 (Figure 7). IB data were more dispersed
lected from the same panel (Figure 5) and having the and poorly correlated with the density (R 2 = 0.274).
same average density showed in fact that the local den- The wide spread in the IB data was most likely related
sity varied considerably and randomly within the cross to the density profile of the produced panels (Figure 5).
section. A very careful mat forming focused to an even In contrast to standard wood fibreboards (which are
distribution of the husk, reduced the warping of panels. characterised by obviously denser surfaces and a low-
Always in concern to the material distribution, a density and much weaker core layer in which the IB
slight asymmetry of the density profile was observed fracture is initiated), the coconut husk boards had a
for both 5 and 12 mm thick panels (Figure 6), which less-defined profile. The fracture during the IB tests
was most likely associated to a different distribution were therefore localised in correspondence of the weak-
of pith and fibres through the panel thickness. In fact est layer, whose actual density, and therefore resistance,
the fine pith powder was inclined to accumulate was more arbitrary. An increasing trend of IB at the

Figure 5. Density profile of three samples collected by the Figure 6. Density profile of a 5 mm panel (dash line) and
same 5 mm thick panel and having the same average density 12 mm panel (solid line) after sanding (each line is the average
(1050 kg m−3). of n = 8 samples).
INTERNATIONAL WOOD PRODUCTS JOURNAL 7

Figure 7. MOE (dash line; cross marker) and MOR (solid line; diamond marker) of 5 mm thick binderless panels made of milled
coconut husk (n = 138 measurements). The green region represents the most suitable density range for the production of binder-
less coconut husk boards with sufficient mechanical properties and low risk of delamination or warping.

increase of the density could however, be observed, in 2002). The lack of highly-densified surfaces, the limited
particular if the average IBs of 5 mm thick panels was length of the milled coconut fibres (1–2 cm), and the
confronted with their average density (Table 1). absence of a suitable thermosetting adhesive were likely
These linear dependencies have been reported as well related to these differences. The binderless panels pro-
for wood-based panels (Kollmann et al. 1975; Deppe duced also showed lower mechanical properties than
and Ernst 1996). the panels produced by van Dam, van den Oever,
The European guidelines for 5 mm thick fibreboards Keijsers (2004) and Snijder et al. (2005) with the
to be used in non-load bearing application and dry high-pressure process followed by cooling. These
environment (EN622-5) recommended MOR > panels were however characterised by much higher
23 N mm−2, MOE > 2700 N mm−2 and IB > densities (1300–1400 kg m−3). Extrapolating the observed
0.65 N mm−2. In relation to the linear regression trends towards this density range the values resulted, as a
lines calculated for 5 mm thick panels, to meet the matter of fact, in good agreement (Figure 7).
minimum requirements for MOR and MOE the den- Thicker coconut panels appeared to have slightly
sity of the coconut husk panels had to be higher than better, even if not significantly higher MOR than thin-
1000 kg m−3 (Figure 7). Above this boundary, the effi- ner panels. Samples of 12 mm in thickness and about
cacy of the developed pressing cycle in avoiding cracks 900 kg m−3 in density showed in fact MOR equal to
and blisters was however considerably reduced. This 19.3 ± 3.1 N mm−2 (n = 10). The achieved bending
lead to the predicament that to produce undamaged properties were in any case not high enough to satisfy
panels the density has to stay below 1000 kg m−3, the EN 622-5 requirements.
while to pass MOR and the MOE in EN 622-5 a density
above 1000 kg m−3 is required. IB requirements were
Thickness swelling
satisfied only in samples with density higher than
900 kg m−3. The thickness swelling of a 5 mm thick panel with an
Coconut husk panels of 5 mm in thickness and average density of 900 kg m−3 was equal to 17.4 ±
between 900 and 1000 kg m−3 in density were however 2.2% (n = 5). For the panel with an average density
able to satisfy the Japanese standard JIS A 5905:2003 equal to 1050 kg m−3 the TS was 12.2 ± 1.2% (n = 10),
mechanical requirements for Type 15 MDF to be used while for a 772 kg m−3 dense panel TS was 21.0 ±
in dry condition (MOR ≥ 15 N mm−2; IB ≥ 2.0% (n = 7). An increase of the TS at the decrease of
0.3 N mm−2), and could therefore be of commercial inter- the panel average density was therefore observed,
est in the Asian market in non-load bearing applications. most likely related to the worsening of the interconnec-
In comparison with wood fibreboards of similar tion between the husk particles. All the results fulfilled
densities, the bending properties of binderless coconut the EN 622-5 requirements for panel thicknesses below
husk boards were clearly poorer (Dunky and Niemz 8 mm (TS < 30%), but only samples with density above
900 kg m−3 fulfilled the JIS A 5905 standards (TS <
17%).
Table 1. Internal bonding (IB) of 5 mm panels at three different For 12 mm thick panels, the TS variation at the
average densities.
change of the density were more pronounced. Panels
Panel Density [kg m−3] IB [N mm−2]
with an average density of 900 kg m−3 showed TS =
1 1082 (±28) 1.50 (±0.33)
2 1003 (±10) 1.17 (±0.15) 18.0 ± 0.9% (n = 10), while for 765 kg m−3 dense panels
3 913 (±23) 0.63 (±0.21) was TS = 46 ± 16% (n = 5). Both the EN 622-5 and the
Note: Mean ± standard deviation are reported; n = 10. JIS A 5905 guidelines have more restricted TS
8 T. BÖGER ET AL.

requirements for thicker boards (TS < 15% and TS < Deppe H-J, Ernst K. 1996. MDF – Mitteldichte Faserplatten.
12%, respectively). The 12 mm thick panels did not Leinfelden-Echterdingen: DRW-Verlag Weinbrenner
thus fulfil the both requirements. The strong drop of GmbH & Co.
Dunky M, Niemz P. 2002. Holzwerkstoffe und Leime.
the TS at the lower densities in 12 mm panels was Heidelberg: Springer Verlag.
most likely related to an insufficient development in FAOSTAT. 2015. Food and agriculture organization of the
innermost layers of the suitable thermal conditions to United Nations statistic division. [accessed 2015 May
activate the self-bonding mechanism. 28]. Available at: http://faostat3.fao.org/faostat-gateway/
go/to/download/P/*/E
Ganchero EG, Manapol P. 2007. Case study – coco technol-
Conclusions ogy: providing livelihood opportunities for poor coconut
farmers through value-adding. United Nations
Binderless panels made of coconut husk of 5 and 12 mm Development Programme, New York.
in thickness were successfully produced in a density Hadinoto R. 1957. Coconut husk is a new raw material for
range between 900 and 1000 kg m−3. A hot pressing board production in copra producing countries. Tech
Inf Circ. 25:1–10.
cycle which permitted an efficient steam pressure release Hashim R, Saari N, Sulaiman O, Sugimoto T, Hiziroglu S,
and working in a pressure range similar to conventional Sato M, Tanaka R. 2010. Effect of particle geometry on
MDF production, was developed. The cycle represented the properties of binderless particleboard manufactured
an improvement with respect to previously reported from oil palm trunk. Mater Des. 31:4251–4257.
technologies, which operated at very high pressure and Kollmann FF, Kuenzi EW, Stamm AJ. 1975. Principles of
included a long and energy wasting cooling phase. The wood science and technology II – wood based materials.
Berlin: Springer Verlag.
final mechanical and physical properties of the 5 mm Mobarak F, Fahmy Y, Augustin H. 1982. Binderless lignocel-
thick panel were not enough to satisfy the European lulose composite from bagasse and mechanism of self-
standard, but were in agreement with the Japanese JIS bonding. Holzforschung. 36:131–135.
A 5905 requirements for Type 15 MDF. The 12 mm Nadhari WNAW, Hashim R, Sulaiman O, Sato M, Sugimoto
thick panels failed however to satisfy the thickness swel- T, Selemat ME. 2013. Utilization of oil palm trunk waste
for manufacturing of binderless particleboard: optimiz-
ling requirements of both standards.
ation study. Bioresources. 8:1675–1696.
Remaining challenges include a method for a mat- Nonaka S, Umemura K, Kawai S. 2013. Characterization of
forming method that avoids uneven distribution of bagasse binderless particleboard manufactured in high-
pith and fibres in the panel. A study on the possibility temperature range. J Wood Sci. 59:50–56.
to increase the bending properties was considered a Okuda N, Sato M. 2004. Manufacture and mechanical prop-
priority for further developments. erties of binderless boards from kenaf core. J Wood Sci.
50:53–61.
Pintiaux T, Viet D, Vandenbossche V, Rigal L, Rouilly A.
2015. Binderless materials obtained by thermo-compres-
Acknowledgments
sive processing of lignocellulosic fibres: a comprehensive
For the support with the processing of the coconut husk and review. BioResources. 10:1915–1963.
manufacturing of the panels, the authors express also their Ramadhas A, Jayaraj S, Muraleedharan C. 2008. Dual fuel
gratitude to Stadtgärtnerei Biel (Biel, Switzerland), Friedli mode operation in diesel engines using renewable fuels:
AG (Burgdorf, Switzerland) and Dieffenbacher GmbH rubber seed oil and coir-pith producer gas. Renew
(Eppingen, Germany). Energy. 33:2077–2083.
Snijder M, Keijsers E, van den Oever MJ, van Dam JE. 2005.
Coir based building and packaging materials. Amsterdam:
Disclosure statement Commen Fund for Commodities.
van Dam JE, van den Oever MJ, Keijsers ER. 2004.
No potential conflict of interest was reported by the authors. Production process for high density high performance
binderless boards from whole coconut husk. Ind Crops
Prod. 20:97–101.
Funding van Dam JE, van den Oever MJ, Teunissen W, Keijsers ER.
The authors express their grateful acknowledgment to the 2004. Process for production of high density/high per-
HILTI Foundation (Schaan, Liechtenstein) for the financial formance binderless boards from whole coconut husk.
support of the present research project. Part 1: lignin as intrinsic thermosetting binder resin. Ind
Crops Prod. 19:207–216.
Youngquist JA, English BE, Scharmer RC, Chow P, Shook
SR. 1994. Literature review on use of nonwood plant fibers
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