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Sound absorption performance of natural fibers and their composites

Article  in  Science China Technological Sciences · August 2012


DOI: 10.1007/s11431-012-4943-1

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SCIENCE CHINA
Technological Sciences
• RESEARCH PAPER • August 2012 Vol.55 No.8: 2278–2283
doi: 10.1007/s11431-012-4943-1

Sound absorption performance of natural fibers and their


composites
YANG WeiDong & LI Yan*
School of Aerospace Engineering and Applied Mechanics, Tongji University, Shanghai 200092, China

Received April 19, 2012; accepted May 25, 2012; published online June 30, 2012

This research aimed to study the sound absorption properties of natural fibers and their reinforced composites. Sound absorp-
tion coefficients of three types of natural fibers, i.e., ramie, flax and jute fibers and their composites were measured by the
two-microphone transfer function technique in the impedance tube. The results were compared with synthetic fibers and their
composites. It was found that both natural fibers and their composites had superior capability of noise reduction. The mul-
ti-scale and hollow lumen structures of natural fibers contributed to the high sound absorption performance. Moreover, the
sound absorption properties of these natural fibers were also calculated by the Delany-Bazley and Garai-Pompoli models. They
showed good agreement with the experimental data. It was concluded that multi-functional composite materials can be made
by natural fibers so that both the mechanical and acoustical functions can be achieved.

natural fiber reinforced composites, sound absorption, impedance tube

Citation: Yang W D, Li Y. Sound absorption performance of natural fibers and their composites. Sci China Tech Sci, 2012, 55: 22782283, doi:
10.1007/s11431-012-4943-1

1 Introduction composites have drawn a lot of attention from material sci-


entists and engineers in recent years due to their good me-
chanical properties, light weight, environmentally friendly
Nowadays noise pollution has become the third pollution
and biodegradable [2, 3]. However, natural fibers, as fibrous
resource that has great adverse influences on the environ-
porous materials, have also been interested in yielding the
ment, human health and economy. How to reduce the dam-
variety of new sound absorption structures in more recent
ages of noise has become an important issue. Generally, the
years [4–7]. As a kind of fibers, natural fibers are supposed
means of controlling noise include active control and pas-
to have the same mechanism for acoustic absorption as oth-
sive control [1]. The former is accomplished by reducing
er conventional synthetic fibrous materials, like glass fiber
the production of noise at the locations of noise sources, but
and mineral wool. The mechanisms of sound absorption in
it can only control the noises of a narrow frequency range.
porous fiber material are basically the viscous effects due to
The passive control is normally achieved by utilizing high
the internal friction between fiber wall and airflow, and
sound absorption materials, which can be used to absorb
thermal losses due to heat transfer among different fibers
noises of a wide frequency range by effectively dissipating
[8].
sound energy on the process of propagation of the sound
Previously, the sound absorption coefficient of a material
wave.
was measured by the well-known standing-wave-ratio
Natural fibers such as ramie, jute, kenaf, etc. reinforced
(SWR) method. However, the SWR method is relatively
time consuming due to the requirements of a single fre-
*Corresponding author (email: liyan@tongji edu.cn)

© Science China Press and Springer-Verlag Berlin Heidelberg 2012 tech.scichina.com www.springerlink.com
Yang W D, et al. Sci China Tech Sci August (2012) Vol.55 No.8 2279

quency operation, a travelling microphone inside the im- acoustic measurements were machined by water jet that
pedance tube, and a method of accurate location of the guaranteed the sample to have superior dimension accuracy.
minimum sound pressure. In recent years, a method, called Plain woven glass and carbon fibers and their composites
transfer function method [9], which calculates the transfer were also prepared in the same way as those of natural fi-
function between the sound pressures at two settled loca- bers for comparison.
tions, Mic.1 and Mic.2 (as shown in Figure 1), has been The impedance tube for the transfer function method was
extensively used. employed to measure the sound absorption coefficients of
Delany and Bazley [10] studied the impedance and wave fibers and composites. The facilities were made by BSWA
propagation properties of fibrous materials in 1970s. They Technology Co., Ltd, as shown in Figure 2. The tests were
normalized these parameters into dimensionless groups and conducted according to ISO10534-2 standard. The meas-
presented simple power-law relations obtained by a large urements are composed of SW422, SW477 and SW499
amount of experimental data of glass fiber and mineral wool. impedance tubes with diameters of 100, 30 and 16 mm for
The empirical model is still a good and fast approximation measuring frequencies from 63–2000, 800–6300 and 2500–
to the theoretical calculations because the model needs only 10000 Hz, respectively. The sound absorption coefficients
one input parameter, the airflow resistivity. In addition, of fibers were measured at frequencies from 63 to 2000 Hz
Garai and Pompoli [11] developed an empirical model due to the edge constraint effects and the difficulties of
based on a number of measurements upon polyester fibers. achieving the dimensional accuracies of the fabrics for
Due to the differences of fiber diameters and the densities of smaller samples [12]. The measurements were conducted at
the matrix materials, they corrected some parameters in frequencies from 63 to 10000 Hz for composites at 25℃
order to apply the calculations of polyester fibers effectively. and 60% relative humidity. The test samples of natural fiber
It should be pointed out that the diameter and density of and synthetic fiber reinforced composites are shown in Fig-
polyester are similar to natural fiber. Thus, using Garai and ure 3.
Pompoli model to predict the sound absorption parameter of
natural fiber might give an accurate result.
In this study, the sound absorption coefficient of natural 3 Results and discussion
fibers, like flax, ramie and jute fiber, and their composites
were studied from both experimental and theoretical. The 3.1 Sound absorption behavior of natural fibers
mechanisms of the sound absorption were proposed. The
results were also compared with those of synthetic fibers, Figure 4 compares the sound absorption coefficients of nat-
which proved that natural fiber composites have superior ural fibers (ramie, flax and jute) with synthetic fibers (car-
acoustic absorption properties and are good candidates for bon and glass fibers). It can be found that jute fiber has the
sound absorption structures.

2 Materials and experiment

Three kinds of plain woven natural fibers which are ramie,


flax and jute fibers were used to study the acoustic absorp-
tion performance. All the natural fiber samples had the
identical thickness of 40 mm for measurements. Three kinds
of natural fibers reinforced epoxy composites were made by
hot press. The fiber volume fractions were around 65% and
the thickness was around 3 mm. The composite samples for

Figure 2 Impedance tube by transfer function technique.

Figure 1 Schematic diagram of instrumentation for the transfer function


method of measuring sound absorption coefficients of natural fiber rein- Figure 3 Acoustic measurement samples of different fibers reinforced
forced composites. Mic.1 and Mic.2 denote two microphones. composites with diameters of 100, 30 and 16 mm, respectively.
2280 Yang W D, et al. Sci China Tech Sci August (2012) Vol.55 No.8

energy; finally, the vibration of air in the bulk materials will


also lead to the vibration of fibers [13].
Figure 6 compares the cross-sections of natural fibers
and synthetic fibers. Figure 6(a) shows the cross-section of
a single sisal fiber (which can be a typical representative of
the structures of natural fibers) and Figure 6(b) shows the
cross-sections of several glass fibers. It is found that a sin-
gle sisal fiber is made up of a bundle of hollow subfibers
that have lumen inside. However, for glass fiber (also a
typical representative for synthetic fibers), each fiber has
the same regular and solid construction. Figure 7 further
indicates the unique structural characteristics of natural
fibers. Therefore, natural fibers are porous fiber materials
which contain many connected open air cavities and those
air cativities might be the major contributors of sound en-
Figure 4 Sound absorption coefficients of natural and synthetic fibers. ergy absorption. The sound wave could propagate by vibra-
tion through the air spaces and inside the lumen of natural
best sound absorption property especially at frequencies fibers, in which the friction effect between cell wall and
above 1000 Hz. The sound absorption coefficient is basi- airflow would transform sound energy into heat. Thus the
cally higher than 0.9. Additionally, the sound absorption unique lumen structure endowed the superior sound
coefficients of flax and ramie fibers are about 0.8 and 0.6 at absorption ability, compared to glass and carbon fibers.
frequencies above 800 Hz, respectively. However, the val- Moreover, by further observing the microstructures of
ues for glass and carbon fibers are overall lower than those natural fibers, it can be realized that natural fiber possesses
of natural fibers. In order to make an easy visual compari- a multi-scale structure as shown in Figure 7. A single sisal
son among the different fibers, the noise reduction coeffi- fiber is made up of a bundle of hollow subfibers. The
cients (NRCs), defined as the arithmetic mean value of cellwall of a subfiber is made up of millions of nano fibrils
sound absorption coefficients at 250, 500, 1000 and 2000 [14]. The nano-sized fibrils would also lead to the extra
Hz, are summarized in Figure 5. It is found that NRCs of vibration, which caused more sound energy dissispation.
ramie, jute and flax are as high as 0.6, 0.65 and 0.65 while
those of glass and carbon are 0.35 and 0.45, respectively. 3.2 Theoretical predication of sound absorption prop-
The mechanism of fibrous materials to absorb sound en- erties of natural fibers
ergy mainly involves three physical processes: Firstly, when
the sound wave transmits into the fibers, the viscous effect The Delany-Bazley empirical model needs the flow resisti-
between fiber frame and numerous air cavities will attenuate
part of sound energy and convert it into heat; secondly, heat
transfer will happen due to temperature distinction between
different fibers and this process will further dissipate sound

Figure 5 Noise reduction coefficient (NRC) comparison of natural and


synthetic fibers. Figure 6 Cross-section morphology of (a) sisal fiber and (b) glass fiber.
Yang W D, et al. Sci China Tech Sci August (2012) Vol.55 No.8 2281

rely on the airflow resistivity values calculated with the


Mechel models, which is expressed by

6.8 (1   )1.296
 , (5)
a 2 3
where  is the viscosity of air (equal to 1.84×105 Pa s),
a is the radius of the fibers and  is the porosity which can
be determined by fiber matrix density and bulk density.
Figure 8 shows that the measured sound absorption coef-
ficient for the jute fiber in the impedance tube tended to
follow the general trend of the theoretical calculations ob-
tained by the predictions of the Delany-Bazley and the
Garai-Pompoli models. The theoretical calculated parame-
ters of natural fibers were shown in Table 1. The calculated
results of the Delany-Bazley model were similar to the pre-
dictions of Garai-Pompoli model, and the sound absorption
Figure 7 Multi-scale and hollow lumen structure of sisal fibers at differ- coefficient curves were consistent with the predictions of
ent magnifications.
the two models. The experimental data were a little larger
than the calculated results of the two models. The experi-
vity and then calculates the complex acoustic impedance, Zc mental sound absorption coefficient of jute fiber at 1600 Hz
and propagation constant, kc both of which can be used to was 0.92, while the values at the same frequency which
further determine the reflection coefficient. were calculated were about 0.98 of those of the two theo-
retical models.
  0 f 
0.754
 0 f 
0.732

Z c   0 c  1  0.0571    j0.087    , (1)
        3.3 Sound absorption behavior of natural fiber rein-
 
forced composites
  f 
0.7
 f 
0.595

kc    1  0.0978  0   j0.189  0   , (2) Figure 9 shows the sound absorption coefficients of these
c       
 

where  0 and c are the density and speed of air media,


respectively,  is the flow resistivity, f is the frequency
and   2f is the angular frequency.
The Garai-Pompoli model was utilized to predict the
flow resistivity, acoustic impedance and sound absorption
coefficient of polyester fibers, the diameters and density of
which are relatively close to those of natural fibers.

  0 f 
0.623
 0 f 
0.660

Z c   0 c  1  0.078    j0.074    , (3)
       
 

  f 
0.53
 f 
0.571

kc    1  0.121  0   j0.159  0  . (4)
c       
  Figure 8 Sound absorption coefficient curves of the jute fiber by experi-
mental results compared with the theoretical predictions of Delany-Bazley
The Delany-Bazley and the Garai-Pompoli models must model and Garai-Pompoli model.

Table 1 Theoretical calculated parameters of natural fibers


Fiber diameter Fiber matrix density Fiber bulk density Calculated porosity Calculated flow resistivity
Natural fibers
(m) (g/cm3) (g/cm3) (%) (Pa s/m2)
Flax 15 1.5 0.341 77.29 83421
Ramie 25 1.5 0.443 70.44 123782
Jute 58 1.37 0.411 70.03 19790
2282 Yang W D, et al. Sci China Tech Sci August (2012) Vol.55 No.8

Figure 9 Sound absorption coefficients of natural fibers (ramie, jute and Figure 10 Sound absorption coefficient of epoxy resin.
flax), and synthetic fibers (glass and carbon fiber) reinforced composites.

Compared to natural fibers, the sound absorption proper-


composites at the frequencies from 63 to 10000 Hz. It is ty of their reinforcing composites apparently decreased.
found that sound absorption properties of natural fiber rein- Natural fibers possess excellent sound absorption property
forced composites are overall better than those of the glass by themselves whereas the hollow lumen and air space
and carbon fiber reinforced composites. Jute fiber rein- would be significantly diminished. The resin would occupy
forced composite has the best sound absorption property some effective volume of airflow and the cavities between
and the sound absorption coefficient can be as high as near- fibers and inside lumens were compressed by the pressure
ly 0.9 at 10000 Hz. It indicates that natural fiber reinforced added during the process of composite manufacturing. Fig-
composites have superior noise reduction capability espe- ure 10 shows the sound absorption properties of epoxy resin
cially at high frequency which would be very beneficial for and it can be seen that the sound absorption behavior of the
the aeronautical applications due to the high sound fre- resin system is very low. Additionally, the sound absorption
quency service environment. The density and porosity of the property largely depends on the frequencies of sound wave.
natural fiber reinforced composites and synthetic fiber rein- The higher the frequency, the shorter the sound wave length
forced composites were measured by underwater weighing and the longer the propagation path of sound wave in the
method and the results were shown in Table 2. It can be composites. Therefore, more dissipation of sound energy
seen that compared to glass and carbon fiber reinforced happens in the composites. This explains why natural fiber
composites, natural fibers (flax, ramie and jute) reinforced composites have the best sound absorption performance at
composites possessed lower density and much higher poros- high frequencies.
ity. Therefore, the unique lumen structures of natural fibers
resulted in the lower density and higher porosity of their
reinforcing composites, which contributed to the more 4 Conclusion
sound energy absorption, thus better acoustic absorption
property. It should be pointed out that all the composites The sound absorption property of natural fibers was superi-
studied appeared the sound absorption trough at 8000 Hz. or to synthetic fibers such as glass and carbon fibers due to
This is because that when the thickness of material is equal their unique hollow and multi scale structures. Natural fiber
to or even multiples of a quarter of incident wavelength, the reinforced composites also possessed better acoustic ab-
sound pressure will be the maximum while the vibration sorption behavior than synthetic fiber reinforced composite,
rate of air particles is zero, which leads to the lowest sound especially at high frequencies, which might be very benefi-
energy loss caused by the viscous effect. cial for the aeronautical applications. The theoretical predi-

Table 2 Density and porosity of natural fiber and synthetic fiber reinforced composites
Reinforcing fibers Density (g/cm3) Porosity (%)
Flax 1.12 17.66
Ramie 1.09 16.78
Jute 1.04 18.26
Glass 2.07 4.08
Carbon 1.55 2.14
Yang W D, et al. Sci China Tech Sci August (2012) Vol.55 No.8 2283

cation values obtained from Garai-Pompoli model and 241–249


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